Related papers: Precision molecular spectroscopy for ground state …
We describe a matter-wave amplifier for vibrational ground state molecules, which uses a Feshbach resonance to first form quasi-bound molecules starting from an atomic Bose-Einstein condensate. The quasi-bound molecules are then driven into…
Coherent manipulation of quantum states is of crucial importance in accurate control of a quantum system. A fundamental goal is coherently transferring the population of a desired state with near-unit fidelity. For this propose, we…
We report the creation and characterization of a near quantum-degenerate gas of polar $^{40}$K-$^{87}$Rb molecules in their absolute rovibrational ground state. Starting from weakly bound heteronuclear KRb Feshbach molecules, we implement…
We demonstrate the transfer of $^{23}$Na$^{40}$K molecules from a closed-channel dominated Feshbach-molecule state to the absolute ground state. The Feshbach molecules are initially created from a gas of sodium and potassium atoms via…
Two-color photoassociation of ground state $^6$Li$^{87}$Rb molecules via the $\mathrm{B}^1\Pi$ electronic state using short pulses near a magnetic Feshbach resonance is studied theoretically. A near-resonant magnetic field is applied to mix…
We report here on the production of an ultracold gas of tightly bound Rb2 molecules in the ro-vibrational triplet ground state, close to quantum degeneracy. This is achieved by optically transferring weakly bound Rb2 molecules to the…
Starting from weakly bound Feshbach molecules, we demonstrate a two-photon pathway to the dipolar ground state of bi-alkali molecules that involves only singlet-to-singlet optical transitions. This pathway eliminates the search for a…
Ultracold paramagnetic and polar diatomic molecules are among the promising systems for quantum simulation of lattice-spin models. Unfortunately, their experimental observation is still challenging. Based on our recent \textit{ab-initio}…
A novel atom-molecule conversion technique has been investigated. Ultracold 85Rb atoms sitting in a DC magnetic field near the 155G Feshbach resonance are associated by applying a small sinusoidal oscillation to the magnetic field. There is…
Stimulated Raman Adiabatic Passage (STIRAP) and its variants, such as multi-state chainwise-STIRAP allow efficiently transferring the populations in multi-state system and have been widely used to prepare ultracold deeply-bound molecules.…
We examine dark quantum superposition states of weakly bound Rb2 Feshbach molecules and tightly bound triplet Rb2 molecules in the rovibrational ground state, created by subjecting a pure sample of Feshbach molecules in an optical lattice…
We propose a process to convert ultracold metastable Cs$_2$ molecules in their lowest triplet state into (singlet) ground state molecules in their lowest vibrational levels. Molecules are first pumped into an excited triplet state, and the…
We report the comprehensive theoretical investigation of the Sr-SrOH system identifying it as a promising route to production of ultracold asymmetric top molecules. Combining high-level ab initio electronic structure calculations with…
We generalize the idea of chainwise stimulated Raman adiabatic passage (STIRAP) [Kuznetsova \textit{et al.} Phys. Rev. A \textbf{78}, 021402(R) (2008)] to a photoassociation-based chainwise atom-molecule system, with the goal of directly…
Recently, the quest for an ultracold and dense ensemble of polar molecules has attracted strong interest. Polar molecules have bright prospects for novel quantum gases with long-range and anisotropic interactions, for quantum information…
We use laser light near-resonant with a molecular bound-to-bound transition to control a magnetic Feshbach resonance in ultracold Fermi gases of $^{40}$K atoms. The spectrum of excited molecular states is measured by applying a laser field…
Stimulated Raman adiabatic passage (STIRAP) offers significant advantages for coherent population transfer between un- or weakly-coupled states and has the potential of realizing efficient quantum gate, qubit entanglement, and quantum…
We consider a method of sub-wavelength superlocalization and patterning of atomic matter waves via a two dimensional stimulated Raman adiabatic passage (2D STIRAP) process. An atom initially prepared in its ground level interacts with a…
We report efficient all-optical creation of an ultracold gas of alkaline-earth-metal dimers, $^{88}\rm{Sr}_2$, in their absolute ground state. Starting with weakly bound singlet molecules formed by narrow-line photoassociation in an optical…
We have converted an ultracold Fermi gas of $^6$Li atoms into an ultracold gas of $^6$Li$_2$ molecules by adiabatic passage through a Feshbach resonance. Approximately $1.5 \times 10^5$ molecules in the least-bound, $v = 38$, vibrational…