English

Ultracold $^{88}\rm{Sr}_2$ molecules in the absolute ground state

Atomic Physics 2021-11-01 v1 Chemical Physics Quantum Physics

Abstract

We report efficient all-optical creation of an ultracold gas of alkaline-earth-metal dimers, 88Sr2^{88}\rm{Sr}_2, in their absolute ground state. Starting with weakly bound singlet molecules formed by narrow-line photoassociation in an optical lattice, followed by stimulated Raman adiabatic passage (STIRAP) via a singlet-dominant channel in the (1)0u+(1)0_u^+ excited potential, we prepare pure samples of more than 5500 molecules in X1Σg+(v=0,J=0)X^1\Sigma_g^+(v=0,J=0). We observe two-body collisional loss rates close to the universal limit for both the least bound and most bound vibrational states in X1Σg+X^1\Sigma_g^+. We demonstrate the enhancement of STIRAP efficiency in a magic-wavelength optical lattice where thermal decoherence is eliminated. Our results pave the way for the use of alkaline-earth-metal dimers for high-precision spectroscopy, and indicate favorable prospects for robust quantum state preparation of ultracold molecules involving closed-shell atoms, as well as molecule assembly in deep optical traps tuned to a magic wavelength.

Keywords

Cite

@article{arxiv.2108.05996,
  title  = {Ultracold $^{88}\rm{Sr}_2$ molecules in the absolute ground state},
  author = {K. H. Leung and E. Tiberi and B. Iritani and I. Majewska and R. Moszynski and T. Zelevinsky},
  journal= {arXiv preprint arXiv:2108.05996},
  year   = {2021}
}
R2 v1 2026-06-24T05:04:54.236Z