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STIRAP (Stimulated Raman Adiabatic Passage) is a powerful laser-based method, usually involving two photons, for efficient and selective transfer of population between quantum states. A particularly interesting feature is the fact that the…

In this paper, a theoretical method for the efficient creation and detection of deeply bound molecules in three-state $\Lambda$-type and five-state M-type molecular systems is proposed. The method is based on the three-state coincident…

Atomic Physics · Physics 2024-03-25 Jiahui Zhang

In this work, we observe a novel resonant mechanism, namely the modulation-induced Feshbach resonance. By applying a far-detuned laser to the cesium D2 transition with intensity modulation, we periodically shake the energy levels of atomic…

Quantum Physics · Physics 2025-12-30 Tongkang Wang , Yuqi Liu , Jundong Wang , Youjia Huang , Wenlan Chen , Zhendong Zhang , Jiazhong Hu

Accurate control of a quantum system is a fundamental requirement in many areas of modern science ranging from quantum information processing to high-precision measurements. A significantly important goal in quantum control is to prepare a…

The technique of stimulated Raman adiabatic passage (STIRAP), which allows efficient and selective population transfer between quantum states without suffering loss due to spontaneous emission, was introduced in 1990 (Gaubatz \emph{et al.},…

Quantum Physics · Physics 2017-04-04 Nikolay V. Vitanov , Andon A. Rangelov , Bruce W. Shore , Klaas Bergmann

Stimulated Raman Adiabatic Passage (STIRAP) is a widely used method for adiabatic population transfer in a multilevel system. In this work, we study STIRAP under novel conditions and focus on the fractional, F-STIRAP, which is known to…

We experimentally demonstrate Cs2 Feshbach molecules well above the dissociation threshold, which are stable against spontaneous decay on the timescale of one second. An optically trapped sample of ultracold dimers is prepared in an l-wave…

Other Condensed Matter · Physics 2008-02-29 S. Knoop , M. Mark , F. Ferlaino , J. G. Danzl , T. Kraemer , H. -C. Naegerl , R. Grimm

The emerging field of ultracold molecules with their rich internal structure is currently attracting a lot of interest. Various methods have been developed to produce ultracold molecules in pre-set quantum states. For future experiments it…

We report on two-photon photoassociation (PA) spectroscopy of ultracold heteronuclear LiRb molecules. This is used to determine the binding energies of the loosely bound levels of the electronic ground singlet and the lowest triplet states…

Quantum Gases · Physics 2017-01-25 Sourav Dutta , Jesús Pérez-Ríos , D. S. Elliott , Yong P. Chen

We discuss a simple scheme for preparing atoms and molecules in an arbitrary preselected coherent superposition of quantum states. The technique, which we call fractional stimulated Raman adiabatic passage ({\it f-STIRAP}), is based upon…

Quantum Physics · Physics 2007-05-23 N. V. Vitanov , K. -A. Suominen , B. W. Shore

In some recent experiments an ultracold gas of $^{40}$K$_2$ (or $^{6}$Li$_2$) molecules has been produced from a degenerate two-component Fermi gas of $^{40}$K (or $^{6}$Li) atoms by adiabatic passage through a Feshbach resonance. The…

Statistical Mechanics · Physics 2007-05-23 Hui Hu , Feng Yuan , Shaojin Qin

We present precision measurements with MHz uncertainty of the energy gap between asymptotic and well bound levels in the electronic ground state X $^1\Sigma_{\mathrm{g}}^+$ of the $^{39}$K$_2$ molecule. The molecules are prepared in a…

Chainwise stimulated Raman adiabatic passage (C-STIRAP) in M-type molecular system is a good alternative in creating ultracold deeply-bound molecules when the typical STIRAP in {\Lambda}-type system does not work due to weak Frank-Condon…

Quantum Physics · Physics 2024-08-06 Jiahui Zhang , Li Deng , Yueping Niu , Shangqing Gong

We report on a resonantly coupled 2(1) - 4 (1) photoassociation resonance in LiRb. This pair of states displays interesting decay physics that hint at interference-like effects caused by two different decay paths. We observe decay to…

Atomic Physics · Physics 2016-12-28 I. C. Stevenson , D. Blasing , Y. P. Chen , D. S. Elliott

We associate Sr atom pairs on sites of a Mott insulator optically and coherently into weakly-bound ground-state molecules, achieving an efficiency above 80\%. This efficiency is 2.5 times higher than in our previous work [S. Stellmer, B.…

Quantum Gases · Physics 2017-07-25 Alessio Ciamei , Alex Bayerle , Chun-Chia Chen , Benjamin Pasquiou , Florian Schreck

We analyse the formation of ultracold 7Li133Cs molecules in the rovibrational ground state through photoassociation into the B1Pi state, which has recently been reported [J. Deiglmayr et al., Phys. Rev. Lett. 101, 133004 (2008)]. Absolute…

Atomic Physics · Physics 2015-03-13 J. Deiglmayr , P. Pellegrini , A. Grochola , M. Repp , R. Côté , O. Dulieu , R. Wester , M. Weidemüller

This paper reviews current experimental and theoretical progress in the study of dipolar quantum gases of ground and meta-stable atoms with a large magnetic moment. We emphasize the anisotropic nature of Feshbach resonances due to coupling…

Atomic Physics · Physics 2015-06-23 Svetlana Kotochigova

We report on the realization of an ultracold mixture of lithium atoms in the ground state and ytterbium atoms in the excited metastable 3P2 state. Such a mixture can support broad magnetic Feshbach resonances which may be utilized for the…

We produce ${^{84}\mathrm{Sr}_2}$ molecules using Bose-enhanced Raman photoassociation. We apply the stimulated Raman adiabatic passage (STIRAP) technique on a Bose-Einstein condensate (BEC) to produce more than $8 \times 10^3$ ultracold…

Quantum Gases · Physics 2017-12-05 Alessio Ciamei , Alex Bayerle , Benjamin Pasquiou , Florian Schreck

We develop a pulse-driven jump protocol to achieve all-optical Raman control of ultracold atomic hyperfine states. By establishing general conditions for adiabatic evolution between quantum states in parameter space, we derive the essential…

Quantum Physics · Physics 2025-04-15 Xin-Xia Jian , Zhi-Jian Zheng , Jun-Jie Jiang , Lin Zhou , Chuan-Cun Shu , Jun He
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