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We investigate a metallic glass-forming (GF) material (Al90Sm10) exhibiting a fragile-strong (FS) glass-formation by molecular dynamics simulation to better understand this highly distinctive pattern of glass-formation in which many of the…

Soft Condensed Matter · Physics 2023-06-01 Hao Zhang , Xinyi Wang , Jiarui Zhang , Hai-Bin Yu , Jack F. Douglas

The fragile-to-strong crossover seems to be a general feature of metallic glass-forming liquids. Here, we study the behavior of shear viscosity, diffusion coefficient and vibrational density of states for…

Soft Condensed Matter · Physics 2019-08-07 René Alvarez Donado , Samuel Cajahuaringa , Alex Antonelli

We study theoretically and numerically the elastic properties of hard sphere glasses, and provide a real-space description of their mechanical stability. In contrast to repulsive particles at zero-temperature, we argue that the presence of…

Soft Condensed Matter · Physics 2015-06-18 E. DeGiuli , E. Lerner , C. Brito , M. Wyart

Because of the negative inclination of the solid-liquid phase separation line in water, ice Ih melts on compression. On further increase in pressure the liquid water transforms into a high density metastable glassy state, characterized by a…

Soft Condensed Matter · Physics 2021-04-22 Saumyak Mukherjee , Biman Bagchi

A model glass with fast and slow processes is studied. The statics is simple and the facilitated slow dynamics is exactly solvable. The main features of a fragile glass take place: Kauzmann transition, Vogel-Fulcher law, Adam-Gibbs relation…

Statistical Mechanics · Physics 2009-11-07 L. Leuzzi , Th. M Nieuwenhuizen

We perform kinetic Monte Carlo simulations of a distinguishable-particle lattice model of structural glasses with random particle interactions. By varying the interaction distribution and the average particle hopping energy barrier, we…

Soft Condensed Matter · Physics 2021-01-04 Chun-Shing Lee , Matteo Lulli , Ling-Han Zhang , Hai-Yao Deng , Chi-Hang Lam

By confining water in nano-pores of silica glass, we can bypass the crystallization and study the pressure effect on the dynamical behavior in deeply supercooled state using neutron scattering. We observe a clear evidence of a cusp-like…

Soft Condensed Matter · Physics 2009-11-11 Li Liu , Sow-Hsin Chen , Antonio Faraone , Chun-Wan Yen , Chung-Yuan Mou

We provide a theoretical perspective on the glass transition in molecular liquids at thermal equilibrium, on the spatially heterogeneous and aging dynamics of disordered materials, and on the rheology of soft glassy materials. We start with…

Statistical Mechanics · Physics 2011-06-22 Ludovic Berthier , Giulio Biroli

Glass transition is a reversible transition that occurs in most amorphous materials. However, the nature of glass transition remains far from being clarified. A key to understand the glass transition is to clarify what determines the glass…

Materials Science · Physics 2025-01-22 Lijian Song , Meng Gao , Juntao Huo , Li-Min Wang , Yuanzheng Yue , Jun-Qiang Wang

We study theoretically and numerically the microscopic cause of the mechanical stability of hard sphere glasses near their maximum packing. We show that, after coarse-graining over time, the hard sphere interaction can be described by an…

Soft Condensed Matter · Physics 2007-05-23 Carolina Brito , Matthieu Wyart

We address the question of the dependence of the fragility of glass forming supercooled liquids on the softness of an interacting potential by performing numerical simulation of a binary mixture of soft spheres with different power n of the…

Soft Condensed Matter · Physics 2007-05-23 Cristiano De Michele , Francesco Sciortino , Antonio Coniglio

Recent ideas based on the properties of assemblies of frictionless particles in mechanical equilibrium provide a perspective of amorphous systems different from that offered by the traditional approach originating in liquid theory. The…

Statistical Mechanics · Physics 2009-07-09 R. Mari , F. Krzakala , J. Kurchan

We analyze a simple dynamical model of glasses, based on the idea that each particle is trapped in a local potential well, which itself evolves due to hopping of neighbouring particles. The glass transition is signalled by the fact that the…

Condensed Matter · Physics 2009-10-28 Jean-Philippe Bouchaud , Alain Comtet , Cécile Monthus

The fragility of a glassforming liquid characterizes how rapidly its relaxation dynamics slow down with cooling. The viscosity of strong liquids follows an Arrhenius law with a temperature-independent barrier height to rearrangements…

Soft Condensed Matter · Physics 2020-08-25 Ekin D. Cubuk , Andrea J. Liu , Efthimios Kaxiras , Samuel S. Schoenholz

We study colloidal particle dynamics of a model glass system using confocal and fluorescence microscopy as the sample evolves from a hard-sphere glass to a liquid with attractive interparticle interactions. The transition from hard-sphere…

Soft Condensed Matter · Physics 2015-05-13 Andrzej Latka , Yilong Han , Ahmed M. Alsayed , Andrew B. Schofield , A. G. Yodh , Piotr Habdas

The reformulation of the mode-coupling theory (MCT) of the liquid-glass transition which incorporates the element of metastability is applied to the hard-sphere system. It is shown that the glass transition in this system is not a sharp one…

Condensed Matter · Physics 2016-08-31 Joonhyun Yeo

We investigate glassy dynamical properties of one component three-dimensional system of particles interacting via pair repulsive potential by the molecular dynamic simulation in the wide region of densities. The glass state is superfragile…

Soft Condensed Matter · Physics 2013-01-11 R. E. Ryltsev , N. M. Chtchelkatchev , V. N. Ryzhov

Understanding glass formation is a challenge because the existence of a true glass state, distinct from liquid and solid, remains elusive: Glasses are liquids that have become too viscous to flow. An old idea, as yet unproven…

We use computer simulations to investigate the static properties of a simple glass-forming fluid in which the positions of a finite fraction of the particles has been frozen in. By probing the equilibrium distribution of the overlap between…

Disordered Systems and Neural Networks · Physics 2015-06-12 Walter Kob , Ludovic Berthier

We report an experimental investigation of the caging motion in a uniformly heated granular fluid, for a wide range of filling fractions, $\phi$. At low $\phi$ the classic diffusive behavior of a fluid is observed. However, as $\phi$ is…

Soft Condensed Matter · Physics 2009-11-11 Pedro M. Reis , Rohit A. Ingale , Mark D. Shattuck