English

The distribution of forces affects vibrational properties in hard sphere glasses

Soft Condensed Matter 2015-06-18 v3

Abstract

We study theoretically and numerically the elastic properties of hard sphere glasses, and provide a real-space description of their mechanical stability. In contrast to repulsive particles at zero-temperature, we argue that the presence of certain pairs of particles interacting with a small force ff soften elastic properties. This softening affects the exponents characterizing elasticity at high pressure, leading to experimentally testable predictions. Denoting P(f)fθeP(f)\sim f^{\theta_e} the force distribution of such pairs and ϕc\phi_c the packing fraction at which pressure diverges, we predict that (i) the density of states has a low-frequency peak at a scale ω\omega^*, rising up to it as D(ω)ω2+aD(\omega) \sim \omega^{2+a}, and decaying above ω\omega^* as D(ω)ωaD(\omega)\sim \omega^{-a} where a=(1θe)/(3+θe)a=(1-\theta_e)/(3+\theta_e) and ω\omega is the frequency, (ii) shear modulus and mean-squared displacement are inversely proportional with δR21/μ(ϕcϕ)κ\langle \delta R^2\rangle\sim1/\mu\sim (\phi_c-\phi)^{\kappa} where κ=22/(3+θe)\kappa=2-2/(3+\theta_e), and (iii) continuum elasticity breaks down on a scale c1/δz(ϕcϕ)b\ell_c \sim1/\sqrt{\delta z}\sim (\phi_c-\phi)^{-b} where b=(1+θe)/(6+2θe)b=(1+\theta_e)/(6+2\theta_e) and δz=z2d\delta z=z-2d, where zz is the coordination and dd the spatial dimension. We numerically test (i) and provide data supporting that θe0.41\theta_e\approx 0.41 in our bi-disperse system, independently of system preparation in two and three dimensions, leading to κ1.41\kappa\approx1.41, a0.17a \approx 0.17, and b0.21b\approx 0.21. Our results for the mean-square displacement are consistent with a recent exact replica computation for d=d=\infty, whereas some observations differ, as rationalized by the present approach.

Keywords

Cite

@article{arxiv.1402.3834,
  title  = {The distribution of forces affects vibrational properties in hard sphere glasses},
  author = {E. DeGiuli and E. Lerner and C. Brito and M. Wyart},
  journal= {arXiv preprint arXiv:1402.3834},
  year   = {2015}
}

Comments

5 pages + 4 pages supplementary information