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In the quest to realize a quantum spin liquid (QSL), magnetic long-range order is hardly welcome. Yet it can offer deep insights into a complex world of strong correlations and fluctuations. Much hope was placed in the cubic pyrochlore…

At low temperatures, Tb$_2$Ti$_2$O$_7$ enters a spin liquid state, despite expectations of magnetic order and/or a structural distortion. Using neutron scattering, we have discovered that in this spin liquid state an excited crystal field…

Strongly Correlated Electrons · Physics 2014-01-16 T. Fennell , M. Kenzelmann , B. Roessli , H. Mutka , J. Ollivier , M. Ruminy , U. Stuhr , O. Zaharko , L. Bovo , A. Cervellino , M. K. Haas , R. J. Cava

We study experimentally and numerically the dynamics of the spin ice material Dy$_2$Ti$_2$O$_7$ in the low temperature ($T$) and moderate magnetic field ($\mathbf{B}$) regime ($T\in[0.1,1.7]K$, $B\in[0,0.3]T$). Our objective is to…

An adiabatic demagnetization process is studied in Gd2Ti2O7, a geometrically frustrated antiferromagnet on a pyrochlore lattice. In contrast to conventional paramagnetic salts, this compound can exhibit a temperature decrease by a factor of…

Strongly Correlated Electrons · Physics 2007-05-23 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , A. I. Golov , I. B. Berkutov , O. A. Petrenko , G. Balakrishnan , M. E. Zhitomirsky

We explore the magnetic properties of Nd$_2$Zr$_2$O$_7$ and Pr$_2$Zr$_2$O$_7$ single crystals subjected to pulsed magnetic fields up to 60 T using magnetization and magnetocaloric-effect (MCE) measurements, with initial temperatures ranging…

Dynamic magnetic properties of $\mathrm{Y_{0.7}Ca_{0.3}MnO_{3}}$ are reported. The system appears to attain local ferromagnetic order at $T_{\mathrm{SRF}} \approx 70$ K. Below this temperature the low field magnetization becomes history…

Materials Science · Physics 2009-10-31 R. Mathieu , P. Nordblad , D. N. H. Nam , N. X. Phuc , N. V. Khiem

We combine two aspects of magnetic frustration, multiferroicity and emergent quasi-particles in spin liquids, by studying magneto-electric monopoles. Spin ice offers to couple these emergent topological defects to external fields, and to…

Strongly Correlated Electrons · Physics 2015-06-24 Ludovic D. C. Jaubert , R. Moessner

We study electron correlations and their impact on magnetic properties of bcc vanadium by a combination of density functional and dynamical mean-field theory. The calculated uniform magnetic susceptibility {in bcc structure} is of Pauli…

Strongly Correlated Electrons · Physics 2023-01-12 A. S. Belozerov , A. A. Katanin , V. I. Anisimov

We discuss magnetization curves of a toy-model trigonal and tetrahedral clusters. Nonlinearity of magnetization with local minimum of differential susceptibility resembling known magnetization plateaus of triangular-lattice and pyrochlore…

Strongly Correlated Electrons · Physics 2019-06-26 V. N. Glazkov

We report the low temperature magnetic properties of Ce$_2$Sn$_2$O$_7$, a rare-earth pyrochlore. Our susceptibility and magnetization measurements show that due to the thermal isolation of a Kramers doublet ground state, Ce$_2$Sn$_2$O$_7$…

Strongly Correlated Electrons · Physics 2016-08-15 Romain Sibille , Elsa Lhotel , Vladimir Pomjakushin , Chris Baines , Tom Fennell , Michel Kenzelmann

The spin ice system Dy$_{2}$Ti$_{2}$O$_{7}$ exhibits strong frequency-dependent spin-freezing at $\sim$ 16 K temperature. Although it has been a matter of discussion for years, the origin of this unusual spin freezing is still unknown. The…

Strongly Correlated Electrons · Physics 2022-04-06 Sheetal , C. S. Yadav

Using muon-spin-relaxation measurements we show that the pyrochlore compound Gd2Ti2O7, in its magnetically orderered phase below ~ 1 K, displays persistent spin dynamics down to temperatures as low as 20 mK. The characteristics of the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Yaouanc , P. Dalmas de Reotier , V. Glazkov , C. Marin , P. Bonville , J. A. Hodges , P. C. M. Gubbens , S. Sakarya , C. Baines

A quantum spin liquid (QSL) is a state of matter characterized by fractionalized quasiparticle excitations, quantum entanglement, and a lack of long-range magnetic order. However, QSLs have evaded definitive experimental observation.…

Strongly Correlated Electrons · Physics 2024-12-31 Sangyun Lee , Andrew J. Woods , Minseong Lee , Shengzhi Zhang , Eun Sang Choi , A. O. Scheie , D. A. Tennant , J. Xing , A. S. Sefat , R. Movshovich

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

Strongly Correlated Electrons · Physics 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

The structure and magnetic properties of rare-earth ions Tm$^{3+}$ kagom\'{e} lattice Tm$_3$Sb$_3$Mg$_2$O$_{14}$ are studied by X-ray diffraction, magnetic susceptibility and muon spin relaxation ($\mu$SR) experiments. The existence of a…

Strongly Correlated Electrons · Physics 2023-10-02 Yanxing Yang , Kaiwen Chen , Zhaofeng Ding , Adrian D. Hillier , Lei Shu

We report the structural and magnetic properties of a quantum magnet PbCuTeO5. The triclinic structure of PbCuTeO5 comprises of alternating layers (ab-planes), in which one layer is composed of S = 1/2 dimer chains and another layer is…

Strongly Correlated Electrons · Physics 2017-05-31 B. Koteswararao , S. P. Chilakalapudi , Aga Shahee , P. V. Srinivasarao , S. Srinath , A. V. Mahajan

We present an experimental study of the quantum spin ice candidate pyrochlore coumpound \przr\ by means of magnetization measurements, specific heat and neutron scattering up to 12 T and down to 60 mK. When the field is applied along the…

We have studied the field induced magnetic structures in the spin liquid Tb$_2$Ti$_2$O$_7$, in a wide temperature (0.3$<$$T$$<$270 K) and field (0$<$$H$$<$7 T) range, by single crystal neutron diffraction with $\bf{H}$ // [110] axis. We…

Strongly Correlated Electrons · Physics 2009-11-13 H. Cao , A. Gukasov , I. Mirebeau , P. Bonville , G. Dhalenne

Using a combination of single-crystal neutron scattering and reverse Monte Carlo refinements, we study the magnetic structure of paramagnetic MnO at a temperature (160\,K) substantially below the Curie-Weiss temperature…

We study the finite temperature properties of the candidate quantum spin ice material Yb$_2$Ti$_2$O$_7$ within the framework of an anisotropic nearest-neighbor spin $1/2$ model on the pyrochlore lattice. Using a combination of finite…

Strongly Correlated Electrons · Physics 2018-05-21 Hitesh J. Changlani