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Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin…

The pyrochlore material Yb2Ti2O7 displays unexpected quasi-two-dimensional (2D) magnetic correlations within a cubic lattice environment at low temperatures, before entering an exotic disordered ground state below T=265mK. We report neutron…

Strongly Correlated Electrons · Physics 2012-02-13 K. A. Ross , L. R. Yaraskavitch , M. Laver , J. S. Gardner , J. A. Quilliam , S. Meng , J. B. Kycia , D. K. Singh , H. A. Dabkowska , B. D. Gaulin

We report high resolution single crystal x-ray diffraction measurements of the frustrated pyrochlore magnet Tb2Ti2O7, collected using a novel low temperature pulsed magnet system. This instrument allows characterization of structural…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , Z. Islam , J. P. Clancy , K. A. Ross , H. Nojiri , Y. H. Matsuda , H. A. Dabkowska , A. D. Dabkowski , B. D. Gaulin

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

The spin ice materials, including Ho2Ti2O7 and Dy2Ti2O7, are rare earth pyrochlore magnets which, at low temperatures, enter a constrained paramagnetic state with an emergent gauge freedom. Remarkably, the spin ices provide one of very few…

Strongly Correlated Electrons · Physics 2014-07-29 Michel J. P. Gingras , Paul A. McClarty

The pyrochlore magnet Tb$_{2}$Ti$_{2}$O$_{7}$ shows a lack of magnetic order to low temperatures and is considered to be a quantum spin liquid candidate. We perform time-domain THz spectroscopy on high quality Tb$_{2}$Ti$_{2}$O$_{7}$…

Strongly Correlated Electrons · Physics 2021-04-21 Xinshu Zhang , Yi Luo , T. Halloran , J. Gaudet , Huiyuan Man , S. M. Koohpayeh , N. P. Armitage

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

High resolution X-ray scattering measurements on single crystal Tb2Ti2O7 reveal finite structural correlations at low temperatures. This geometrically frustrated pyrochlore is known to exhibit a spin liquid, or cooperative paramagnetic…

Disordered Systems and Neural Networks · Physics 2009-11-13 J. P. C. Ruff , B. D. Gaulin , J. P. Castellan , K. C. Rule , J. P. Clancy , J. Rodriguez , H. A. Dabkowska

We report an analysis of neutron diffraction from single crystals of the spin-liquid pyrochlore Tb2Ti2O7 under the application of magnetic fields along the crystallographic $[110]$ direction. Such a perturbation has been shown to destroy…

Strongly Correlated Electrons · Physics 2009-11-17 J. P. C. Ruff , B. D. Gaulin , K. C. Rule , J. S. Gardner

We report a positive muon spin relaxation and rotation (\muSR) study of the quantum spin ice materials Yb2Ti2O7 and Yb2Sn2O7 focusing on the low field response. In agreement with earlier reports, data recorded in small longitudinal fields…

Strongly Correlated Electrons · Physics 2015-09-24 A. Maisuradze , P. Dalmas de Reotier , A. Yaouanc , A. Forget , C. Baines , P. J. C. King

In the pyrochlore compounds, Tb$_2$Ti$_2$O$_7$ and Tb$_2$Sn$_2$O$_7$, only the Tb$^{3+}$ ions are magnetic. They exhibit quite abnormal -- and, in view of their chemical similarity, strikingly different -- magnetic behaviour, as probed by…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apetrei , I. N. Goncharenko , R. Moessner

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

Strongly Correlated Electrons · Physics 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

The intrinsic noncollinear spin patterns in rare-earth pyrochlore are physically interesting, hosting many emergent properties, e.g. spin ice and monopole-type excitation. Recently, the magnetic monopole excitation of spin ice systems was…

Materials Science · Physics 2015-12-18 Lin Lin , Y. L. Xie , J. -J. Wen , Shuai Dong , Z. B. Yan , J. -M. Liu

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with…

Strongly Correlated Electrons · Physics 2018-10-03 S. K. Takahashi , A. Arsenault , C. Mauws , A. M. Hallas , C. Sarkis , K. A. Ross , C. R. Wiebe , M. Tachibana , G. M. Luke , T. Imai

The spin-liquid phase of two highly frustrated pyrochlore magnets Gd2Ti2O7 and Gd2Sn2O7 is probed using electron spin resonance in the temperature range 1.3 - 30 K. The deviation of the absorption line from the paramagnetic position \nu…

Strongly Correlated Electrons · Physics 2013-05-29 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , P. Bonville , G. Jasmin - Le Bras , O. A. Petrenko

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

Quantum spin liquids are highly entangled ground states of quantum systems with emergent gauge structure, fractionalized spinon excitations, and other unusual properties. While these features clearly distinguish quantum spin liquids from…

Strongly Correlated Electrons · Physics 2013-06-18 Lucile Savary , Leon Balents

Static and dynamical properties of the magnetic moment system of pyrochlore compound Tb2Ti2O7 with strong magnetic frustration, have been investigated down to the temperature T=0.4 K by neutron scattering on a single crystal sample. The…

In their recent communication (Phys. Rev. B 64, 060406(R) (2001)) Cornelius and Gardner have reported the results of magnetization and susceptibility studies on single crystals of the pyrochlore Ho2Ti2O7. The observed field dependence of…

Strongly Correlated Electrons · Physics 2009-11-07 O. A. Petrenko , M. R. Lees , G. Balakrishnan