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Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

Elastic and inelastic neutron scattering studies have been carried out on the pyrochlore magnet Ho2Ti2O7. Measurements in zero applied magnetic field show that the disordered spin ice ground state of Ho2Ti2O7 is characterized by a pattern…

Strongly Correlated Electrons · Physics 2016-08-05 J. P. Clancy , J. P. C. Ruff , S. R. Dunsiger , Y. Zhao , H. A. Dabkowska , J. S. Gardner , Y. Qiu , J. R. D. Copley , T. Jenkins , B. D. Gaulin

Spin ices, frustrated magnetic materials analogous to common water ice, are exemplars of high frustration in three dimensions. Recent experimental studies of the low-temperature properties of the paradigmatic Dy$_2$Ti$_2$O$_7$ spin ice…

Statistical Mechanics · Physics 2016-01-19 P. Henelius , T. Lin , M. Enjalran , Z. Hao , J. G. Rau , J. Altosaar , F. Flicker , T. Yavors'kii , M. J. P. Gingras

The ground states of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$, sensitively depending on the small off-stoichiometry parameter $x$, have been studied by specific heat measurements using well characterized samples. Single…

Strongly Correlated Electrons · Physics 2016-02-09 M. Wakita , T. Taniguchi , H. Edamoto , H. Takatsu , H. Kadowaki

We present a simple model for a description of magnetization processes in rare-earth tetraborides. The model is based on the coexistence of two subsystems, and namely, the spin subsystem described by the Ising model and the electronic…

Strongly Correlated Electrons · Physics 2015-05-18 Pavol Farkašovský , Hana Čenčariková , Slavomir Mataš

We report the results of low-temperature measurements of the specific heat Cp(T), ac susceptibility chi(T) and 23Na nuclear magnetic resonance NMR of Na2V3O7. At liquid He temperatures Cp(T)/T exhibits broad field-dependent maxima, which…

Strongly Correlated Electrons · Physics 2009-11-11 J. L. Gavilano , E. Felder , D. Rau , H. R. Ott , P. Millet , F. Mila , T. Cichorek , A. C. Mota

Recent experimental results have emphasized two aspects of Tb2Ti2O7 which have not been taken into account in previous attempts to construct theories of Tb2Ti2O7: the role of small levels of structural disorder, which appears to control the…

Strongly Correlated Electrons · Physics 2016-05-04 M. Ruminy , L. Bovo , E. Pomjakushina , M. K. Haas , U. Stuhr , A. Cervellino , R. J. Cava , M. Kenzelmann , T. Fennell

We studied the field-induced magnetic structures of the Tb2Ti2O7 pyrochlore by single-crystal neutron diffraction with a magnetic field applied along a [110] axis, focusing on the influence of a small misalignment. Both induced magnetic…

Strongly Correlated Electrons · Physics 2010-11-10 A. P. Sazonov , A. Gukasov , I. Mirebeau , H. Cao , P. Bonville , B. Grenier , G. Dhalenne

A quantum melting of the spin ice is proposed for pyrochlore-lattice magnets Pr$_2TM_2$O$_7$ ($TM=$Ir, Zr, and Sn). The quantum superexchange Hamiltonian having a nontrivial magnetic anisotropy is derived in the basis of atomic non-Kramers…

Strongly Correlated Electrons · Physics 2010-07-26 Shigeki Onoda , Yoichi Tanaka

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…

The pyrochlore iridates have become ideal platforms to unravel fascinating correlated and topolog?ical phenomena that stem from the intricate interplay among strong spin-orbit coupling, electronic correlations, lattice with geometric…

The pyrochlore compounds Ho2Ti2O7 and Dy2Ti2O7 show an exotic form of magnetism called the spin ice state, resulting from the interplay between geometrical frustration and ferromagnetic coupling. A fascinating feature of this state is the…

Materials Science · Physics 2013-09-11 D. P. Leusink , F. Coneri , M. Hoek , S. Turner , H. Idrissi , G. Van Tendeloo , H. Hilgenkamp

The pyrochlore oxides Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$ are well studied spin ice systems and have shown the evidences of magnetic monopole excitations. Unlike these, Dy$_{2}$Zr$_{2}$O$_{7}$ is reported to crystallize in a…

Strongly Correlated Electrons · Physics 2020-08-26 Sheetal , Anzar Ali , Sarita Rajput , Yogesh Singh , Tulika Maitra , C. S. Yadav

The description and detection of unconventional magnetic states such as spin liquids is a recurring topic in condensed matter physics. While much of the efforts have traditionally been directed at geometrically frustrated antiferromagnets,…

Strongly Correlated Electrons · Physics 2018-05-25 L. Bovo , M. Twengström , O. A. Petrenko , T. Fennell , M. J. P. Gingras , S. T. Bramwell , P. Henelius

Magnetic susceptibility, specific heat, and muon spin relaxation ($\mu$SR) measurements have been performed on a newly synthesized three-dimensional sandglass-type lattice Tm$_3$SbO$_7$, where two inequivalent sets of non-Kramers Tm$^{3+}$…

Strongly Correlated Electrons · Physics 2022-05-25 Yan-Xing Yang , Yao Wang , Zhao-Feng Ding , Adrian D. Hillier , Lei Shu

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

1T-tantalum disulphide (1T-TaS2) is a promising material to realize quantum spin liquid state and fractional excitations. Here, we take a closer look on the temperature dependent magnetic susceptibility of 1T-TaS2 at low magnetic fields to…

Strongly Correlated Electrons · Physics 2022-07-28 Sudip Pal , S. B. Roy

At low temperatures, a spin ice enters a Coulomb phase - a state with algebraic correlations and topologically constrained spin configurations. In Ho2Ti2O7, we have observed experimentally that this process is accompanied by a non-standard…

We report the thermodynamic and muon spin relaxation ($\mu$SR) evidences for a possible gapless spin liquid in Tm$_{3}$Sb$_{3}$Zn$_{2}$O$_{14}$, with the rare-earth ions Tm$^{3+}$ forming a two-dimensional kagom\'{e} lattice. We extract the…

Strongly Correlated Electrons · Physics 2018-11-09 Zhaofeng Ding , Yanxing Yang , Jian Zhang , Cheng Tan , Zihao Zhu , Gang Chen , Lei Shu

Low-temperature states of polycrystalline samples of a frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by specific heat, magnetic susceptibility, and neutron scattering experiments. We have found that this…

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