Related papers: Nonlinear Optical Response Functions of Mott Insul…
We present a theoretical study of the nonlinear magneto-optical shift conductivity in the surface states of the prototypical topological insulator Bi$_2$Se$_3$ under a perpendicular quantizing magnetic field. By describing the electronic…
We present a systematic theoretical study of the multi-photon nonlinear optical absorption properties of a $\text{GaAs/A}{{\text{l}}_{x}}\text{G}{{\text{a}}_{1-x}}\text{As}$ based quantum well (QW) structure with Morse confinement potential…
The nonlinear optical response of materials under high-intensity electromagnetic fields is key to advancing THz optical technologies. This study introduces a theoretical approach to estimate the nonlinear refractive index coefficient n2 of…
Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…
We investigate the role of short-ranged electron-electron interactions in a paradigmatic model of three dimensional topological insulators, using dynamical mean-field theory and focusing on non magnetically ordered solutions. The…
The non-linear response of infinite periodic solids to homogenous electric fields and collective atomic displacements is discussed in the framework of density functional perturbation theory. The approach is based on the 2n + 1 theorem…
The optical properties of a spherical topological insulator embedded concentrically in a single-electron system consisting of a core-shell GaAs quantum dot are analyzed, when the system is under a uniform external magnetic field. The…
Exciton effects on conjugated polymers and the resulting optical nonlinearities are investigated in soliton lattice systems. The magnitude of the THG at the 10 percent doping increases by the factor about 10^2 from that of the neutral…
We employ dynamical density-matrix renormalization group (DDMRG) and field-theory methods to determine the frequency-dependent optical conductivity in one-dimensional extended, half-filled Hubbard models. The field-theory approach is…
Two-photon absorption (TPA) spectra of push-pull chromophores are described in terms of a two-state model accounting for electron-vibration coupling. Vibrations have two main effects in TPA spectra. The most obvious one is the appearance of…
We have observed the characteristic temperature dependence of the intermolecular phonon spectrum in the organic dimer Mott insulator kappa-(ET)2Cu2(CN)3 exhibiting a dielectric anomaly at 30 K. The anomalous spectral narrowing of the 55…
We have studied the nonlinear conductivity of two-dimensional Coulomb glasses. We have used a Monte Carlo algorithm to simulate the dynamic of the system under an applied electric field $E$. We found that in the nonlinear regime the site…
We perform a theoretical study of nonlinear optical isolator devices based on coupled microcavities with gain and loss. Using coupled-mode theory, we derive a correspondence between the boundary of asymptotic stability in the nonlinear…
Based on the Bethe-Salpeter equation eigenstates, we present a first-principles many-body formalism for calculating the two-photon absorption (TPA) coefficient of semiconductors. We apply this formalism to calculate the TPA spectra of MoS2…
We compute the time-resolved photoemission spectrum after photo-doping in a two-dimensional Mott-Hubbard insulator. We find that the relaxation rate of high-energy photo-doped electrons in the paramagnetic phase scales with the strength of…
Recently, the field of strongly correlated electrons has begun an intense search for a correlation induced topological insulating phase. An example is the quadratic band touching point which arises in a checkerboard lattice at half-filling,…
High Harmonic Generation (HHG) promises to provide insight into ultrafast dynamics and has been at the forefront of attosecond physics since its discovery. One class of materials that demonstrate HHG are Mott insulators whose electronic…
High-temperature superconductivity emerges in the CuO$_2$ plane upon doping a Mott insulator. To ascertain the influence of Mott physics plus short-range correlations, we solve a three-band copper-oxide model in the charge-transfer regime…
First-principles dynamical CPA (Coherent-Potential Approximation) for electron correlations has been developed further by taking into account higher-order dynamical corrections with use of the asymptotic approximation. The theory is applied…
We investigate experimentally the ultrafast changes in the spectral response of the Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl ($\kappa$-Cl) upon photodoping with intense excitation at 1.6 eV and probing with continuum pulses…