Related papers: Nonlinear Optical Response Functions of Mott Insul…
Non-perturbative phenomena in four-wave mixing spectra of semiconductors are studied using the exact solution of a widely used phenomenological non-linear equation of motion of the exciton polarization. It is shown that Coulomb interaction,…
We report an experimental and theoretical investigation of a system whose dynamics is dominated by an intricate interplay between three key concepts of modern physics: topology, nonlinearity, and spontaneous symmetry breaking. The…
Improving the efficiency of photothermal (PT) therapies and photoacoustic (PA) imaging at the microscopic scale hinges on developing multiphoton-absorbing photothermal molecules or contrast agents that operate in the near-infrared (NIR)…
Recently, Tao and Mo (TM) proposed an accurate all-purpose nonempirical meta-generalized gradient approximation (meta-GGA). The exchange part was derived from the density matrix approximation, while the correlation part is based on a…
In this paper, we examined the effects of proximity-induced interactions such as Rashba spin-orbit coupling (SOC) and effective Zeeman fields (EZFs) on the optical spectrum of $n$-type and $p$-type monolayer (ML)-MoS$_2$. The optical…
We study the influence of third-harmonic generation (THG) and negative frequency polarization terms in the self-phase modulation (SPM) of short and intense pulses in Kerr media. We find that THG induces additional symmetric lobes in the SPM…
We have previously demonstrated that in the context of two-dimensional (2D) coherent electronic spectroscopy measured by phase modulation and phase-sensitive detection, an \emph{incoherent} nonlinear response, due to pairs of…
Strong two-photon absorption (TPA) in monolayer MoS2 is demonstrated in contrast to saturable absorption (SA) in multilayer MoS2 under the excitation of femtosecond laser pulses in the near infrared region. MoS2 in the forms of monolayer…
High-harmonic generation (HHG) in strongly correlated Mott insulators is investigated using exact diagonalization and time-dependent density-matrix propagation of a laser-driven one-dimensional Hubbard chain. By projecting onto equilibrium…
Nonlinear optical responses are often used as a probe for studying electronic properties of materials. For topological materials, studies so far focused on the photogalvanic electric current, which requires breaking inversion symmetry. In…
The nonlinear response of stochastic models obeying a master equation is calculated up to fifth-order in the external field thus extending the third-order results obtained earlier (G. Diezemann, Phys. Rev. E{\bf 85}, 051502 (2012)). For…
Dynamical mean-field theory is employed to calculate the electronic charge reconstruction of multilayered inhomogeneous devices composed of semi-infinite metallic lead layers sandwiching barrier planes of a strongly correlated material…
$\beta$-Ga$_2$O$_3$ is an ultra-wide bandgap semiconductor and is thus expected to be optically transparent to light of sub-bandgap wavelengths well into the ultraviolet. Contrary to this expectation, it is found here that free electrons in…
Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…
We studied the pressure dependence of the room-temperature infrared reflectivity of (TMTTF)_2AsF_6 along all three optical axes. This anisotropic organic compound consists of molecular stacks with orbital overlap along the a direction; due…
We report a systematic investigation of both three-photon absorption (3PA)spectra and wavelength dispersions of Kerr-type nonlinear refraction in wide-gap semiconductors. The Z-scan measurements are recorded for both ZnO and ZnS with…
We study the optical response of a Mott Hubbard system in the framework of the half--filled Extended Hubbard Model using the Density Matrix Renormalization Group (DMRG) method. We discuss the appearance of excitonic features inside the…
We theoretically investigate the magneto-optical (MO) properties of monolayer (ML) transition metal dichalcogenides (TMDs) in the presence of external electrical and quantizing magnetic fields and of the proximity-induced exchange…
Nonlinear photomagnetization is a process by which an oscillating electric field induces a static magnetization. We show that all 32 crystallographic point groups admit such spin polarization using circularly polarized electric fields to…
We study the effect of Coulomb interaction between two oppositely doped low-dimensional tJ model systems. We exactly show that, in the one-dimensional case, an arbitrarily weak interaction leads to the formation of charge neutral…