Related papers: Optical pumping and vibrational cooling of molecul…
All conventional methods to laser-cool atoms rely on repeated cycles of optical pumping and spontaneous emission of a photon by the atom. Spontaneous emission in a random direction is the dissipative mechanism required to remove entropy…
We report on a generic cooling technique for atoms trapped in optical lattices. It consists in modulating the lattice depth with a proper frequency sweeping. This filtering technique removes the most energetic atoms, and provides with the…
We study the quantum dynamics of an ultracold atomic gas in a deep optical lattice within an optical high-$Q$ resonator. The atoms are coherently illuminated with the cavity resonance tuned to a blue vibrational sideband, so that photon…
Sympathetic cooling with ultracold atoms and atomic ions enables ultralow temperatures in systems where direct laser or evaporative cooling is not possible. It has so far been limited to the cooling of other microscopic particles, with…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
Laser cooling and trapping of atoms and atomic ions has led to numerous advances including the observation of exotic phases of matter, development of exquisite sensors and state-of-the-art atomic clocks. The same level of control in…
We propose an optical pumping scheme to prepare trapped $\mathrm{AlH}^+$ molecules in a pure state, the stretched hyperfine state $\lvert F=\frac{7}{2},\, m_F=\frac{7}{2}\rangle$ of the rovibronic ground manifold $\lvert…
In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…
We propose a generic approach to nonresonant laser cooling of atoms/molecules in a bistable optical cavity. The method exemplifies a photonic version of Sisyphus cooling, in which the matter-dressed cavity extracts energy from the particles…
We predict that it is possible to cool rotational, vibrational and translational degrees of freedom of molecules by coupling a molecular dipole transition to an optical cavity. The dynamics is numerically simulated for a realistic set of…
Atomic-resolution-imaging approaches for single molecules, such as coherent x-ray diffraction at free-electron lasers, require the delivery of high-density beams of identical molecules. However, even very cold beams of biomolecules…
We present a study of Sisyphus cooling of molecules: the scattering of a single-photon remove a substantial amount of the molecular kinetic energy and an optical pumping step allow to repeat the process. A review of the produced cold…
The continuous pumping of atoms into a Bose-Einstein condensate via spontaneous emission from a thermal reservoir is analyzed. We consider the case of atoms with a three-level $\Lambda$ scheme, in which one of the atomic transitions has a…
The rich internal structure and long-range dipole-dipole interactions establish polar molecules as unique instruments for quantum-controlled applications and fundamental investigations. Their potential fully unfolds at ultracold…
Cold supersonic beams of molecules can be slowed down using a switched sequence of electrostatic field gradients. The energy to be removed is proportional to the mass of the molecules. Here we report deceleration of YbF, which is 7 times…
Carbon monoxide molecules in their electronic, vibrational, and rotational ground state are highly attractive for trapping experiments. The optical or ac electric traps that can be envisioned for these molecules will be very shallow,…
We create a dark optical lattice structure using a blue detuned laser field coupling an atomic ground state of total angular momentum F simultaneously to two excited states with angular momenta F and F-1, or F and F+1. The atoms are trapped…
Photonic molecules - particular systems composed of coupled optical resonators - emulate the behavior of complex physical systems exhibiting discrete energy levels. In this work, we present a novel photonic molecule composed of two strongly…
Cooling of molecules via free-space dissipative scattering of photons is thought not to be practicable due to the inherently large number of Raman loss channels available to molecules and the prohibitive expense of building multiple…
We report on the creation of bosonic NaCs molecules in their absolute rovibrational ground state via stimulated Raman adiabatic passage. We create ultracold gases with up to 22,000 dipolar NaCs molecules at a temperature of 300(50) nK and a…