Related papers: Optical pumping and vibrational cooling of molecul…
Laser cooling of atomic motion enables a wide variety of technological and scientific explorations using cold atoms. Here we focus on the effect of laser cooling on the photons instead of on the atoms. Specifically, we show that…
Many theoretical and laboratory studies predict H2 to be formed in highly excited ro-vibrational states. The consequent relaxation of excited levels via a cascade of infrared transitions might be observable in emission from suitable…
Ultracold molecules confined in optical lattices or tweezer traps can be used to process quantum information and simulate the behaviour of many-body quantum systems. Molecules offer several advantages for these applications. They have a…
Cooling a range of molecules to ultracold temperatures (<1 mK) is a difficult but important challenge in molecular physics and chemistry. Collective cavity cooling of molecules is a promising method that does not rely on molecular energy…
Photoassociation of two ultracold rubidium atoms and the subsequent formation of stable molecules in the singlet ground and lowest triplet states is investigated theoretically. The method employs laser pulses inducing transitions via…
Atoms in spatially dependent light fields are attracted to local intensity maxima or minima depending on the sign of the frequency difference between the light and the atomic resonance. For light fields confined in open high-Q optical…
We propose to repeatedly load laser-cooled molecules into optical tweezers, and transfer them to storage states that are rotationally excited by two additional quanta. Collisional loss of molecules in these storage states is suppressed, and…
A cold atomic gas with an inverted population on a transition coupled to a field mode of an optical resonator constitutes a generic model of a laser. For quasi-continuous operation, external pumping, trapping and cooling of the atoms is…
We make use of an inhomogeneous electrostatic dipole field to impart a quantum-state-dependent deflection to a pulsed beam of OCS molecules, and show that those molecules residing in the absolute ground state, $X ^1\Sigma^+$, $\ket{00^00}$,…
We report on a general method for the rapid production of quantum degenerate gases. Using 174Yb, we achieve an experimental cycle time as low as (1.6-1.8) s for the production of Bose-Einstein condensates (BECs) of (0.5-1) x 10^5 atoms.…
We propose a new method for the production of ultracold molecular ions. This method utilizes sympathetic cooling due to the strong collisions between appropriately chosen molecular ions and laser-cooled neutral atoms to realize ultracold,…
We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…
A new physical implementation for quantum computation is proposed. The vibrational modes of molecules are used to encode qubit systems. Global quantum logic gates are realized using shaped femtosecond laser pulses which are calculated…
Polarized atomic ensembles play a crucial role in precision measurements. We demonstrate a novel method of creating atomic polarization in an alkali vapor in a continuous-wave regime. The method relies on a combination of optical pumping by…
We utilize the dark state in a {\Lambda}-type three-level system to cool an ensemble of 85Rb atoms in an optical lattice [Morigi et al., Phys. Rev. Lett. 85, 4458 (2000)]. The common suppression of the carrier transition of atoms with…
We analyze the formation of Rb_2 molecules with short photoassociation pulses applied to a cold Rb-85 sample. A pump laser pulse couples a continuum level of the ground electronic state X ^1\Sigma_{g}^+ with bound levels in the 0_{u}^+…
We study a single incoherently pumped atom moving within an optical high-Q resonator in the strong coupling regime. Using a semiclassical description for the atom and field dynamics, we derive a closed system of differential equations to…
The general idea that optical radiation may cool matter was put forward by Pringsheim already in 1929. Doppler cooling of dilute atomic gases is an extremely successful application of this concept, and more recently anti-Stokes cooling in…
We use a $^{87}\text{Rb}$ atomic vapor, suitable for an optically-pumped magnetometer (OPM) in Earth-field conditions, to study the noise properties of three strategies for generating pulsed optical pumping. We compare a frequency-modulated…
We describe the generation and properties of a cryogenic beam of $^7$Li$_2$ dimers from sublimation of a neon matrix where lithium atoms have been implanted via laser ablation of solid precursors of metallic lithium or lithium hydride…