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Low-energy electron collisions with O$_2$ molecules are studied using the fixed-bond R-matrix method. In addition to the O$_2$ ${X}^3\Sigma_{g}^-$ ground state, integrated cross sections are calculated for elecron collisions with the…

Chemical Physics · Physics 2008-12-18 Motomichi Tashiro , Keiji Morokuma , Jonathan Tennyson

We report on measurements of the collisional properties of a mixture of $^{133}$Cs and $^{87}$Rb atoms in a magnetic trap at $\mu\mathrm{K}$ temperatures. By selectively evaporating the Rb atoms using a radio-frequency field, we achieved…

Soft Condensed Matter · Physics 2009-11-10 M. Anderlini , E. Courtade , M. Cristiani , D. Cossart , D. Ciampini , C. Sias , O. Morsch , E. Arimondo

We report bunching, slowing, and acceleration of a supersonically cooled beam of diatomic hydroxyl radicals (OH). \textit{In situ} observation of laser-induced fluorescence along the beam propagation path allows for detailed…

Atomic Physics · Physics 2009-11-10 J. R. Bochinski , Eric R. Hudson , H. J. Lewandowski , Jun Ye , Gerard Meijer

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…

The experimental characterization of scattering resonances in low energy collisions has proven to be a stringent test for quantum chemistry calculations. Previous measurements on the NO-H$_2$ system at energies down to $10$ cm$^{-1}$…

We present measurements and calculations of the trap loss rate for laser cooled Rb atoms confined in either a magneto-optic or a magnetic quadrupole trap when exposed to a room temperature background gas of Ar. We study the loss rate as a…

We develop an analytic model of thermal state-to-state rotationally inelastic collisions of asymmetric-top molecules with closed-shell atoms in electric fields, and apply it to the Ar--H$_2$O collision system. The predicted cross sections…

Chemical Physics · Physics 2010-01-05 Mikhail Lemeshko , Bretislav Friedrich

Scattering and ionizing cross sections and rates are calculated for ultracold collisions between metastable helium atoms using a fully quantum-mechanical close-coupled formalism. Homonuclear collisions of the bosonic ${}^{4}$He$^{*}…

Atomic Physics · Physics 2019-07-03 D. G. Cocks , I. B. Whittingham , G. Peach

We present a rigorous theoretical study of low-temperature collisions of polyatomic molecular radicals with ^1S_0 atoms in the presence of an external magnetic field. Accurate quantum scattering calculations based on ab initio and scaled…

Atomic Physics · Physics 2011-03-07 T. V. Tscherbul , H-G. Yu , A. Dalgarno

We report a combined experimental and theoretical study of collision-induced dipolar relaxation in a cold spin-polarized gas of atomic nitrogen (N). We use buffer gas cooling to create trapped samples of 14N and 15N atoms with densities…

Atomic Physics · Physics 2011-03-07 T. V. Tscherbul , J. Klos , A. Dalgarno , B. Zygelman , Z. Pavlovic , M. T. Hummon , H-I Lu , E. Tsikata , J. M. Doyle

We experimentally demonstrate cooling of trapped ions by collisions with co-trapped, higher mass neutral atoms. It is shown that the lighter $^{39}$K$^{+}$ ions, created by ionizing $^{39}$K atoms in a magneto-optical trap (MOT), when…

Atomic Physics · Physics 2017-03-23 Sourav Dutta , Rahul Sawant , S. A. Rangwala

Ultracold collisions of LiO molecules in the $^{2}\Pi_{3/2}$ ground state are considered, under the influence of either an external magnetic or electric field. Inelastic collisions are shown to be suppressed in the presence of modest…

Atomic Physics · Physics 2020-09-16 Lucie D. Augustovičová , John L. Bohn

Cold chemical reactions between laser-cooled Ca^+ ions and Rb atoms were studied in an ion-atom hybrid trap. Reaction rate constants were determined in the range of collision energies <E_{coll}>/k_B = 20 mK-20 K. The lowest energies were…

We compute the rotational quenching rates of the first 81 rotational levels of ortho- and para-H2CO in collision with ortho- and para-H2, for a temperature range of 10-300 K. We make use of the quantum close-coupling and coupled-states…

Solar and Stellar Astrophysics · Physics 2015-06-15 Laurent Wiesenfeld , Alexandre Faure

We report the measurement of collision rate coefficient for collisions between ultracold Cs atoms and low energy Cs+ ions. The experiments are performed in a hybrid trap consisting of a magneto-optical trap (MOT) for Cs atoms and a Paul…

Atomic Physics · Physics 2020-08-20 Sourav Dutta , S. A. Rangwala

We consider the cold bosonic ensemble trapped by a helical interference pattern in the optical \textit{loop} scheme. This rotating helical potential is produced by the two slightly detuned counter propagating Laguerre-Gaussian laser beams…

Atomic Physics · Physics 2012-07-17 A. Yu. Okulov

A continuously operated electrostatic trap for polar molecules is demonstrated. The trap has a volume of ~0.6 cm^3 and holds molecules with a positive Stark shift. With deuterated ammonia from a quadrupole velocity filter, a trap density of…

Chemical Physics · Physics 2007-05-23 T. Rieger , T. Junglen , S. A. Rangwala , P. W. H. Pinkse , G. Rempe

We experimentally and theoretically study the continuous accumulation of cold atoms from a magneto-optical trap (MOT) into a finite depth trap, consisting in a magnetic quadrupole trap dressed by a radiofrequency (RF) field. Chromium atoms…

The vibrational quenching cross sections and corresponding low-temperature rate constants for the v = 1 and v = 2 states of CN- colliding with He and Ar atoms have been computed ab initio using new three dimensional potential energy…

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