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We report studies of the Yb$^{3+}$ site distribution in Er$^{3+}$ co-doped upconverting alkaline earth fluoride nanoparticles using high-resolution absorption measurements. Similar to bulk crystals, Yb$^{3+}$ single ion cubic (O$_h$), and…

Materials Science · Physics 2020-04-30 Sangeetha Balabhadra , Michael F. Reid , Vladimir Golovko , Jon-Paul R. Wells

Efficient detection of single optical centers in solids is essential for quantum information processing, sensing, and single-photon generation applications. In this work, we use radio-frequency (RF) reflectometry to electrically detect the…

We report the quantum efficiency of photoluminescence processes of Er optical centers as well as the thermal quenching mechanism in GaN epilayers prepared by metal-organic chemical vapor deposition. High resolution infrared spectroscopy and…

Materials Science · Physics 2016-11-29 V. X. Ho , T. V. Dao , H. X. Jiang , J. Y. Lin , J. M. Zavada , S. A. McGill , N. Q. Vinh

Strongly bound excitons confined in two-dimensional (2D) semiconductors are dipoles with a perfect in-plane orientation. In a vertical stack of semiconducting 2D crystals, such in-plane excitonic dipoles are expected to efficiently couple…

We present a systematic experimental study along with theoretical modeling of the energy transfer in an ensemble of closely-packed CdTe colloidal nanocrystals identified as the F\"orster resonant energy transfer (FRET). We prove that at low…

Mesoscale and Nanoscale Physics · Physics 2015-12-22 Feng Liu , A. V. Rodina , D. R. Yakovlev , A. A. Golovatenko , A. Greilich , E. D. Vakhtin , A. Susha , A. L. Rogach , Yu. G. Kusrayev , M. Bayer

In this review we discuss several fundamental processes taking place in semiconductor nanocrystals (quantum dots, QDs) when their electron subsystem interacts with electromagnetic (EM) radiation. The physical phenomena of light emission and…

Mesoscale and Nanoscale Physics · Physics 2021-01-12 Vladimir A. Burdov , Mikhail I. Vasilevskiy

The elastic scattering cross section measured at energies $E\lesssim 10$ MeV/nucleon for some light heavy-ion systems having two identical cores like $^{16}$O+$^{12}$C exhibits an enhanced oscillatory pattern at the backward angles. Such a…

Nuclear Theory · Physics 2021-07-22 Nguyen Tri Toan Phuc , Nguyen Hoang Phuc , Dao. T. Khoa

Ce3+ doped SrS phosphors with a charge-compensating Na+ for light-emitting diode (LED) applications have been successfully synthesized via a solid-state reaction method, which can be indexed to rock-salt-like crystal structures of Fm-3m…

Materials Science · Physics 2021-11-24 Shuqin Chang , Jipeng Fu , Xuan Sun , Guangcan Bai , Guoquan Liu , Kaina Wang , Ligang Xu , Qi Wei , Thomas Meier , Mingxue Tang

Electron transfer (ET) between primary electron donors and acceptors is modeled in the photosystem II reaction center (RC). Our model includes (i) two discrete energy levels associated with donor and acceptor, interacting through a…

It has been demonstrated in previous experimental and computational work that doping CeO2 with transition metals is an effective way of tuning its properties. However, each previous study on CeO2 doping has been limited to a single or a few…

Materials Science · Physics 2020-12-14 Zhao Liua , Hongyang Ma , Charles C. Sorrell , Pramod Koshy , Judy N. Hart

The nucleation, distribution and composition of erbium embedded in a SiO$_2$-Si layer were studied with High Resolution Transmission Electron Microscopy (HRTEM), Electron Energy Loss Spectroscopy (EELS), Energy Filtered TEM (EFTEM),…

This study investigates the mechanisms underlying ultrafast cross-luminescence observed in BaF$_2$ crystals doped with LaF$_3$. We identified an ultrafast luminescent component with a decay time of approximately 150 ps, which emerges under…

The luminescence of fifteen representative Eu$^{2+}$-doped phosphors used for white-LED and scintillation applications is studied through a Constrained Density Functional Theory. Transition energies and Stokes shift are deduced from…

Materials Science · Physics 2017-09-20 Yongchao Jia , Anna Miglio , Samuel Poncé , Masayoshi Mikami , Xavier Gonze

Chalcogenide-based optical phase change materials (OPCMs) exhibit a large contrast in refractive index when reversibly switched between their stable amorphous and crystalline states. OPCMs have rapidly gained attention due to their…

We report the transport characteristics of both electrons and holes through narrow constricted crystalline Si "wall-like" long-channels that were surrounded by a thermally grown SiO2 layer. Importantly, as a result of the existence of fixed…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 C. S. Mayberry , Danhong Huang , G. Balakrishnan , C. Kouhestani , N. Islam , S. R. J. Brueck , A. K. Sharma

We investigated the Li+ ion incorporation in Ba2GdNbO6:Eu3+ perovskite by atomistic simulations based on energy minimization. We predicted the most probable sites occupied by Eu3+ and Li+ ions and the related charge-compensation mechanisms…

Dye sensitised nanocrystalline solar cells (Gr\"{a}tzel cells) have achieved solar-to-electrical energy conversion efficiencies of 12% in diffuse daylight. The cell is based on a thin film of dye-sensitised nanocrystalline TiO$_2$…

Condensed Matter · Physics 2015-06-24 A Kambili , A B Walker , F Qiu , A C Fisher , A D Savin , L M Peter

Embedded Si and Ge nanocrystals (NCs) in wide band-gap matrices are studied theoretically using an atomistic pseudopotential approach. From small clusters to large NCs containing on the order of several thousand atoms are considered.…

Materials Science · Physics 2007-11-27 C. Bulutay

Resonant energy transfer mechanisms have been observed in the sensitized luminescence of solids, in quantum dots and in molecular nanostructures, and they also play a central role in light harvesting processes in photosynthetic organisms.…

Quantum Physics · Physics 2009-11-07 Brendon Lovett , John H. Reina , Ahsan Nazir , Beeneet Kothari , Andrew Briggs

The understanding of depletion layers is of major importance to control the optical and electronic properties of metal oxide (MO) nanocrystals (NCs). Here, we show that depletion layer engineering is the main mechanism of photodoping of MO…

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