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The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

Atomic Physics · Physics 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu

We use extreme-ultraviolet interferometry to measure the phase of high-order harmonic generation from transiently aligned CO2 molecules. We unambiguously observe a reversal in phase of the high order harmonic emission for higher harmonic…

Atomic Physics · Physics 2009-11-13 Xibin Zhou , Robynne Lock , Wen Li , Nick Wagner , Margaret. M. Murnane , Henry C. Kapteyn

Electron quantum path interferences in strongly laser-driven aligned molecules and their dependence on the molecular alignment is an essential open problem in strong-field molecular physics. Here, we demonstrate an approach which provides…

Experiments have shown that the internal vibrational state of a molecule can affect the intensity of high harmonic light generated from that molecule. This paper presents a model which explains this modulation in terms of interference…

Atomic Physics · Physics 2015-05-13 Zachary B. Walters , Stefano Tonzani , Chris H. Greene

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

Accurate molecular imaging via high-order harmonic generation relies on comparing the harmonic emission from a molecule and an adequate reference system. However, an ideal reference atom with the same ionization properties as the molecule…

Atomic Physics · Physics 2015-05-28 Elmar V. van der Zwan , Manfred Lein

We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

Based upon our previous works (Eur.Phys.J.D 6, 319(1999); Chin.Phys.Lett. 18, 236(2001)), we develop a classical approach to calculate the high-order harmonic generation of the laser driven atoms and molecules. The Coulomb singularities in…

Atomic Physics · Physics 2007-05-23 Chaohong Lee , Yiwu Duan , Wing-Ki Liu , Jian-Min Yuan , Lei Shi , Xiwen Zhu , Kelin Gao

We investigate the orientation dependence of high-order harmonic generation (HHG) from H$_2^+$ with different internuclear distances irradiated by intense laser fields both numerically and analytically. The calculated molecular HHG spectra…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jie Liu , Bambi Hu

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

Quantum Physics · Physics 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

We show that the dependence of high-order harmonic generation (HHG) on the molecular orientation can be understood within a theoretical treatment that does not involve the strong field of the laser. The results for H_2 show excellent…

Atomic Physics · Physics 2009-11-10 B. Zimmermann , M. Lein , J. M. Rost

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

Atomic Physics · Physics 2009-11-10 Manfred Lein , Jan M. Rost

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

The laser interaction with an electron-positron-ion mixed plasma is studied, from the perspective of the associated high-order harmonic generation. For an idealized mixed plasma which is assumed with a sharp plasma-vacuum interface and…

Plasma Physics · Physics 2021-01-20 W. L. Zhang , T. Grismayer , K. M. Schoeffler , R. A. Fonseca , L. O. Silva

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

We develop the strong-field approximation for high-order harmonic generation in hydrogen molecules, including the vibrational motion and the laser-induced coupling of the lowest two Born-Oppenheimer states in the molecular ion that is…

Atomic Physics · Physics 2009-11-13 C. C. Chirila , M. Lein

In the present paper, we investigate the high-order harmonic generation (HHG) from diatomic molecules with large internuclear distance using a strong field approximation (SFA) model. We find that the hump and dip structure emerges in the…

Atomic Physics · Physics 2009-11-13 Y. J. Chen , J. Liu
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