Vibrational interference of Raman and high-harmonic generation pathways
Atomic Physics
2015-05-13 v1
Abstract
Experiments have shown that the internal vibrational state of a molecule can affect the intensity of high harmonic light generated from that molecule. This paper presents a model which explains this modulation in terms of interference between different vibrational states occurring during the high harmonic process. In addition, a semiclassical model of the continuum electron propagation is developed which connects with rigorous treatments of the electron-ion scattering.
Cite
@article{arxiv.0908.0896,
title = {Vibrational interference of Raman and high-harmonic generation pathways},
author = {Zachary B. Walters and Stefano Tonzani and Chris H. Greene},
journal= {arXiv preprint arXiv:0908.0896},
year = {2015}
}