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Using first-principles calculations, we show that the magnetic properties of a two-dimensional antiferromagnetic transition-metal surface are modified on the atomic scale by the adsorption of small organic molecules. We consider benzene…

Materials Science · Physics 2015-06-16 Nuala M. Caffrey , Paolo Ferriani , Simone Marocchi , Stefan Heinze

The exchange interactions and magnetic structure in layered system CuMnO2 (mineral crednerite) and in nonstoichiometric system Cu1.04Mn0.96O2, with triangular layers distorted due to orbital ordering of the Mn3+ ions, are studied by…

Strongly Correlated Electrons · Physics 2014-01-21 A. V. Ushakov , S. V. Streltsov , D. I. Khomskii

The 5d pyrochlore oxide superconductor Cd2Re2O7 (CRO) has attracted significant interest as a spin-orbit-coupled metal (SOCM) that spontaneously undergoes a phase transition to an odd-parity multipole phase by breaking the spatial inversion…

Strongly Correlated Electrons · Physics 2023-09-18 Daigorou Hirai , Atsuhito Fukui , Hajime Sagayama , Takumi Hasegawa , Zenji Hiroi

We present transport and thermal data for the quadruple-perovskites MCu3(Ti1-xRux)4O12 where 0 < x < 1. A metal-insulator transition (MIT) occurs for Ru concentrations x~0.75. At the same time, the Cu2+ antiferromagnetic state is destroyed…

Materials Science · Physics 2009-11-10 A. P. Ramirez , G. Lawes , D. Li , M. A. Subramanian

We study Mn substitution for Ti in BaTiO3 with and without compensating oxygen vacancies using density functional theory (DFT) in combination with dynamical mean field theory (DMFT). We find strong charge and spin fluctuations. Without…

Materials Science · Physics 2018-09-12 Subhasish Mandal , R. E. Cohen , K. Haule

The p-electrons of carbon in the interstitial compound Fe3C hybridize with the Fe d-band and enhance the valence electron concentration of Fe from 8 to 8.67. At this concentration, substitutional 3d transition metals and alloys exhibit…

Materials Science · Physics 2007-05-23 E. Duman , M. Acet , E. F. Wassermann , J. P. Itie , F. Baudelet , O. Mathon , S. Pascarelli

We report on a combined experimental and theoretical study on CrI3 single crystals by employing the polarization dependence of resonant inelastic X-ray scattering (RIXS). Our investigations reveal multiple Cr 3d orbital splitting (dd…

We have investigated dielectric properties in a series of crystals of $R$MnO$_{3}$ ($R$ is a rare earth ion) under magnetic fields and quasihydrostatic pressure. We have found that ferroelectric phase appeared in GdMnO$_3$ crystal below…

Strongly Correlated Electrons · Physics 2009-11-10 H. Kuwahara , K. Noda , J. Nagayama , S. Nakamura

In an externally applied magnetic field, ultra-pure crystals of the bilayer compound Sr$_3$Ru$_2$O$_7$ undergo a metamagnetic transition below a critical temperature, $T^*$, which varies as a function of the angle between the magnetic field…

Strongly Correlated Electrons · Physics 2015-05-13 S. Raghu , A. Paramekanti , E. -A. Kim , R. A. Borzi , S. Grigera , A. P. Mackenzie , S. A. Kivelson

The magnetic and electronic modifications induced at the interfaces in (SrMnO$_{3}$)$_{n}$/(LaMnO$_{3}$)$_{2n}$ superlattices have been investigated by linear and circular magnetic dichroism in the Mn L$_{2,3}$ x-ray absorption spectra.…

We have developed the crystal-field approach with strong electron correlations, extended to the Quantum Atomistic Solid-State theory (QUASST), as a physically relevant theoretical model for the description of electronic and magnetic…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. Radwanski , Z. Ropka

We have performed x-ray linear and circular magnetic dichroism experiments at the Mn L2,3-edge of the La0.7Sr0.3MnO3 ultra thin films. Our measurements show that the antiferromagnetic (AF) insulating phase is stabilized by the interfacial…

Strongly Correlated Electrons · Physics 2009-07-29 C. Aruta , G. Ghiringhelli , V. Bisogni , L. Braicovich , N. B. Brookes , A. Tebano , G. Balestrino

We report on detailed structural, electronic and magnetic studies of GdMn$_{1-x}$Cr$_x$O$_3$ for Cr doping levels 0 $\le$ $x$ $\le$ 1. In the solid solutions, the Jahn-Teller distortion associated with Mn$^{3+}$ ions gives rise to major…

The structural, magnetic, and electronic properties of NdFe$_{0.5}$Mn$_{0.5}$O$_3$ have been studied in detail using bulk magnetization, neutron/x-ray diffraction and first principles density functional theory calculations. The material…

Strongly Correlated Electrons · Physics 2017-10-25 Ankita Singh , A. Jain , Avijeet Ray , B. Padmanabhan , S. M. Yusuf , T. Maitra , V. K. Malik

The rare-earth nitrides form a series of structurally simple $intrinsic$ ferromagnetic semiconductors, a rare class of both fundamental interest and application potential. Within the series there is a wide range of magnetic properties…

The crystal structure and the magnetism of BaMn$_2$O$_3$ have been studied by thermodynamic and by diffraction techniques using large single crystals and powders. BaMn$_2$O$_3$ is a realization of a $S = 5/2$ spin ladder as the magnetic…

Strongly Correlated Electrons · Physics 2015-05-20 M. Valldor , O. Heyer , A. C. Komarek , A. Senyshyn , M. Braden , T. Lorenz

We employed {\it in-situ} pulsed laser deposition (PLD) and angle-resolved photoemission spectroscopy (ARPES) to investigate the mechanism of the metal-insulator transition (MIT) in NdNiO$_3$ (NNO) thin films, grown on NdGaO$_3$(110) and…

Strongly Correlated Electrons · Physics 2015-07-16 R. S. Dhaka , Tanmoy Das , N. C. Plumb , Z. Ristic , W. Kong , C. E. Matt , N. Xu , K. Dolui , E. Razzoli , M. Medarde , L. Patthey , M. Shi , M. Radovic , Joel Mesot

The role of rare-earth (R) ions on the magnetodielectric (MD) coupling is always intriguing and markedly different for different systems. Although many reports are available concerning this aspect in frustrated 3d-transition metal oxides,…

Strongly Correlated Electrons · Physics 2019-11-04 Tathamay Basu , Vincent Caignaert , Somnath Ghara , Xianglin Ke , Alain Pautrat , Stephan Krohns , Alois Loidl , Bernard Raveau

Transmittance of the colossal magnetoresistive compound Nd_0.5Sr_0.5MnO_3 showing metal-insulator phase transition has been studied by means of the submm- and mm-wavelength band spectroscopy. An unusually high transparency of the material…

Condensed Matter · Physics 2016-08-31 S. Zvyagin , A. Angerhofer , K. V. Kamenev , L. -C. Brunel , G. Balakrishnan , D. McK. Paul

The crystal field splitting and d bandwidth of the 3d transition metal monoxides MnO, FeO, CoO and NiO are analyzed as a function of pressure within density functional theory. In all four cases the 3d bandwidth is significantly larger than…

Strongly Correlated Electrons · Physics 2015-05-14 Luke Shulenburger , Sergey Y. Savrasov , R E Cohen