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We report results of structural, magnetic and transport properties of single crystal CaRu1-xCrxO3 (0≤x≤0.36) and SrRu1-xCrxO3 (0≤x≤0.30). Cr substitution as low as x=0.08 drives CaRu1-xCrxO3 from the paramagnetic…

Strongly Correlated Electrons · Physics 2007-05-23 V. Durairaj , E. Elhami , S. Chikara , X. N. Lin , A. Douglass , G. Cao P. Schlottmann , E. S. Choi , R. P. Guertin

In intermetallic compounds with zero-orbital momentum ($L=0$) the magnetic anisotropy and the electronic band structure are interconnected. Here, we investigate this connection on divalent Eu and trivalent Gd intermetallic compounds. We…

Ilmenites $AB$O$_3$ provide a platform for electron correlation and magnetism on alternatively stacked honeycomb layers of edge-sharing $A$O$_6$ or $B$O$_6$ octahedra. When $A$ and $B$ are $3d$ transition metals, strong electron correlation…

Strongly Correlated Electrons · Physics 2024-02-12 Seong-Hoon Jang , Yukitoshi Motome

We have investigated the dielectric anomalies associated with spin ordering transitions in the tetragonal spinel Mn$_3$O$_4$, using thermodynamic, magnetic, and dielectric measurements. We find that two of the three magnetic ordering…

Materials Science · Physics 2007-10-16 R. Tackett , G. Lawes , B. C. Melot , M. Grossman , E. S. Toberer , R. Seshadri

The ground-state orbital occupancy of the Ru$^{4+}$ ion in Ca$_{2-x}$La$_x$RuO$_4$ [x=0, 0.05(1), 0.07(1) and 0.12(1)] was investigated by performing X-ray absorption spectroscopy (XAS) in the vicinity of the O K edge as a function of angle…

Strongly Correlated Electrons · Physics 2019-02-13 D. Pincini , L. S. I. Veiga , C. D. Dashwood , F. Forte , M. Cuoco , R. S. Perry , P. Bencok , A. T. Boothroyd , D. F. McMorrow

We have performed photoemission and soft x-ray absorption studies of pyrochlore-type Ru oxides, namely, the filling-control system Sm$_{2-x}$Ca$_x$Ru$_2$O$_7$ and the bandwidth-control system Sm$_{2-x}$Bi$_x$Ru$_2$O$_7$, which show…

Strongly Correlated Electrons · Physics 2009-11-11 J. Okamoto , S. -I. Fujimori , T. Okane , A. Fujimori , M. Abbate , S. Yoshii , M. Sato

The Mn-terminated (001) surface of the stable anti-ferromagnetic insulating phase of cubic perovskite CaMnO$_3$ is found to undergo a magnetic reconstruction consisting on a spin-flip process at surface: each Mn spin at the surface flips to…

Materials Science · Physics 2009-10-31 Alessio Filippetti , Warren E. Pickett

One way to induce insulator to metal transitions in the spin-orbit Mott insulator Sr2IrO4 is to substitute iridium with transition metals (Ru, Rh). However, this creates intriguing inhomogeneous metallic states, which cannot be described by…

Strongly Correlated Electrons · Physics 2021-09-08 Véronique Brouet , Paul Foulquier , Alex Louat , François Bertran , Patrick Le Fèvre , Julien E. Rault , Dorothée Colson

Topological spin textures in frustrated intermetallics hold great promise for spintronics applications. However, understanding their origin and properties remains a significant challenge due to competing and often long-range interactions…

We use the self-interaction corrected local spin-density approximation to investigate the ground state valency configuration of transition metal (TM = Mn, Co) impurities in n- and p-type ZnO. We find that in pure Zn1-xTMxO, the localized…

Materials Science · Physics 2009-11-11 L. Petit , T. C. Schulthess , A. Svane , W. M. Temmerman , Z. Szotek , A. Janotti

The apparent metal-insulator transition is observed in a high quality two-dimensional electron system (2DES) in the strained Si quantum well of a Si/Si_{1-x}Ge_x heterostructure with mobility \mu=1.9 x 10^5 cm^2/Vs at density n=1.45 x…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 K. Lai , W. Pan , D. C. Tsui , S. A. Lyon , M. Muhlberger , F. Schaffler

Using x-ray absorption spectroscopy at the Rh-L_2,3, Co-L_2,3, and Fe-L_2,3 edges, we find a valence state of Co^2+/Rh^4+ in Ca3CoRhO6 and of Fe^3+/Rh^3+ in Ca3FeRhO6. X-ray magnetic circular dichroism spectroscopy at the Co-L_2,3 edge of…

Strongly Correlated Electrons · Physics 2008-05-15 T. Burnus , Z. Hu , Hua Wu , J. C. Cezar , S. Niitaka , H. Takagi , C. F. Chang , N. B. Brookes , H. -J. Lin , L. Y. Jang , A. Tanaka , K. S. Liang , C. T. Chen , L. H. Tjeng

The magnetic properties of the ferromagnetic semiconductor In0.98Mn0.02As were characterized by x-ray absorption spectroscopy and x-ray magnetic circular dichroism. The Mn exhibits an atomic-like L2,3 absorption spectrum that indicates that…

Materials Science · Physics 2009-11-10 P. T. Chiu , B. W. Wessels , D. J. Keavney , J. W. Freeland

Non-resonant Raman spectroscopy in the hard X-ray regime has been used to explore the electronic structure of the first two members of the Ruddlesden-Popper series Sr$_{n+1}$Ir$_n$O$_{3n+1}$ of iridates. By tuning the photon energy transfer…

We investigated the magnetic phase diagram of single crystals of SrNdFeO$_{4}$ by measuring the magnetic properties, the specific heat and the dielectric permittivity. The system has two magnetically active ions, Fe$^{3+}$ and Nd$^{3+}$.…

Materials Science · Physics 2015-06-05 J. M. Hwang , E. S. Choi , H. D. Zhou , Y. Xin , J. Lu , P. Schlottmann

Strong Coulomb repulsion and spin-orbit coupling are known to give rise to exotic physical phenomena in transition metal oxides. Initial attempts to investigate systems where both of these fundamental interactions are comparably strong,…

First-principles density-functional theory calculations show switching magnetization by 90 degree can be achieved in ultrathin BFO film by applying external electric-field. Up-spin carriers appear to the surface with positive field while…

Materials Science · Physics 2013-02-01 Hong-Jian Feng

Ultra-clean crystals of Sr$_3$Ru$_2$O$_7$ undergo a metamagnetic transition at low temperatures. This transition shows a strong anisotropy in the applied field direction with the critical field $H_c$ ranging from $\sim 5.1$T for $H\perp c$…

Strongly Correlated Electrons · Physics 2010-02-26 Mark H. Fischer , Manfred Sigrist

Structural phase transformations of [110] electric field cooled Pb(Mg1/3Nb2/3)O3-30%PbTiO3 (PMN-30%PT) crystals have been performed by x-ray diffraction in a field-cooled (FC) condition. A phase sequence of…

Materials Science · Physics 2009-11-11 Hu Cao , Feiming Bai , Naigang Wang , Jiefang Li , D. Viehland , Guangyong Xu , Gen Shirane

We study the structural evolution of Sr$_3$Ir$_2$O$_7$ as a function of pressure using x-ray diffraction. At a pressure of 54 GPa at room temperature, we observe a first-order structural phase transition, associated with a change from…

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