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We report on a Ni L$_{2,3}$ edges x-ray absorption spectroscopy (XAS) study in $R$NiO$_3$ perovskites. These compounds exhibit a metal to insulator ($MI$) transition as temperature decreases. The L$_{3}$ edge presents a clear splitting in…

Strongly Correlated Electrons · Physics 2016-08-16 C. Piamonteze , F. M. F. de Groot , H. C. N. Tolentino , A. Y. Ramos , N. E. Massa , J. A. Alonso , M. J. Martínez-Lope

We investigate the interplay between Coulomb driven orbital order and octahedral distortions in strongly correlated Mott insulators due to orbital dilution, i.e., doping by metal ions without an orbital degree of freedom. In particular, we…

Strongly Correlated Electrons · Physics 2020-07-30 Wojciech Brzezicki , Filomena Forte , Canio Noce , Mario Cuoco , Andrzej M. Oleś

Spin-orbit Mott insulators with the $t_{2g}^5$ electron configuration are promising platforms for the Kitaev spin liquid, yet fine-tuning of their crystal structures is essential to suppress non-Kitaev interactions. Here, we investigate the…

Strongly Correlated Electrons · Physics 2026-04-13 Yuya Haraguchi , Hiroko Aruga Katori , Kenji Ishii , Hakuto Suzuki

The pursuit of efficient spin-polarization in quaternary Heusler alloys with the general formula $XX'YZ$ (where X, $X'$, and Y are transition metals and Z is a p-block element), has been a subject of significant scientific interest. While…

We point out the high physical correctness of the use and the concept of the crystal-field approach, even if is used to metallic magnetic materials of transition-metal 3d/4f/5f compounds. We discuss the place of the crystal-field theory in…

Strongly Correlated Electrons · Physics 2008-10-08 R. J. Radwanski , Z. Ropka

Using resonant x-ray diffraction, we observe an easy c-axis collinear antiferromagnetic structure for the bilayer Sr$_3$Ir$_2$O$_7$, a significant contrast to the single layer Sr$_2$IrO$_4$ with in-plane canted moments. Based on a…

Strongly Correlated Electrons · Physics 2012-12-11 J. W. Kim , Y. Choi , Jungho Kim , J. F. Mitchell , G. Jackeli , M. Daghofer , J. van den Brink , G. Khaliullin , B. J. Kim

Correlations between the localized and conductive spins/charges have been the central issue of various fascinating quantum phenomena found on itinerant electron systems. Here, the obvious multiplet structures are presented on the Mn 2$p$ to…

The coercivity of La$_{1-x}$Sr$_x$MnO$_3$ thin films can be enhanced by Ru substitution for Mn. In order to elucidate its mechanism, we performed soft x-ray absorption and magnetic circular dichroism measurements at the Ru M$_{2,3}$ and Mn…

We present first-principles based density functional theory calculations of the electronic and magnetic structure of CrO2 with 3d (Ti through Cu) and 4d (Zr through Ag) substitutional impurities. We find that the half-metallicity of CrO2…

Materials Science · Physics 2015-05-28 M. E. Williams , H. Sims , D. Mazumdar , W. H. Butler

We report results of a magnetic and transport study of SrRu1-xMnxO3, i.e., Mn doped SrRuO3. The Mn doping drives the system from the itinerant ferromagnetic state (TC=165 K for x=0) through a quantum critical point at xc=0.39 to an…

Strongly Correlated Electrons · Physics 2009-11-10 G. Cao , S. Chikara , X. N. Lin , E. Elhami , V. Durairaj , P. Schlottmann

Magnetic control of correlated spin systems is central to the development of next-generation spin-based technologies. Rare-earth orthoferrites provide an interesting platform in which exchange coupling between rare-earth 4f and…

The crystal structure of hexagonal-Sr0.6Ba0.4MnO3 allows various competing superexchange interactions, leading to intriguing magnetic properties. Local structural changes modify overlapping between Mn and oxygen ions with temperature.…

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

A promising route to tailoring the electronic properties of quantum materials and devices rests on the idea of orbital engineering in multilayered oxide heterostructures. Here we show that the interplay of interlayer charge imbalance and…

In order to study the magnetic and crystal structures in the Nd{1-x}Sr{x}MnO{3} system, we have peformed neutron diffraction measurements on melt-grown polycrystalline samples with 0.49 < x < 0.75. As a function of hole concentration x, the…

Strongly Correlated Electrons · Physics 2009-10-31 R. Kajimoto , H. Yoshizawa , H. Kawano , H. Kuwahara , Y. Tokura , K. Ohoyama , M. Ohashi

We use transport and neutron-scattering measurements to show that a magnetic-field-induced transition from noncollinear to collinear spin arrangement in adjacent CuO_{2} planes of lightly electron-doped Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4}…

Superconductivity · Physics 2009-11-10 A. N. Lavrov , H. J. Kang , Y. Kurita , T. Suzuki , Seiki Komiya , J. W. Lynn , S. -H. Lee , Pengcheng Dai , Yoichi Ando

Using x-ray absorption spectroscopy at the Ru-$L_{2,3}$ edge we reveal that the Ru$^{4+}$ ions remain in the $S$=1 spin state across the rare 4d-orbital ordering transition and spin-gap formation. We find using local spin density…

We demonstrate sensitivity of the Mn 3d valence states to strain in the ferromagnetic semiconductors (Ga,Mn)As and (Al,Ga,Mn)As, using x-ray magnetic circular dichroism (XMCD). The spectral shape of the Mn $L_{2,3}$ XMCD is dependent on the…

We report the results of neutron diffraction, ac and dc magnetization, heat-capacity, complex permittivity, and pyrocurrent measurements on an oxide, Li3NiRuO5, hitherto not paid much attention in the literature, except for a previous…

Strongly Correlated Electrons · Physics 2017-05-09 Sanjay Kumar Upadhyay , Kartik K Iyer , S. Rayaprol , V. Siruguri , E. V. Sampathkumaran

Polycrystalline Nd2Ru2O7 samples have been prepared and examined using a combination of structural, magnetic, and electrical and thermal transport studies. Analysis of synchrotron X-ray and neutron diffraction patterns suggests some site…