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We have utilized the resonant x-ray diffraction technique at the Mn L-edge in order to directly compare magnetic and orbital correlations in the Mn sub-lattice of Pr0.6Ca0.4MnO3. The resonant line shape is measured below T_OO ~ 240 K at the…

Strongly Correlated Electrons · Physics 2009-11-10 K. J. Thomas , J. P. Hill , Y-J. Kim , S. Grenier , P. Abbamonte , L. Venema , A. Rusydi , Y. Tomioka , Y. Tokura , D. F. McMorrow , M. van Veenendaal

We report resonant x-ray scattering data of the orbital and magnetic ordering at low temperatures at the Mn $L_{\rm 2,3}$ edges in \lsmo. The orderings display complex energy features close to the Mn absorption edges. Systematic modeling…

We report a x-ray resonant diffraction study of the perovskite Pr0.6Ca0.4MnO3. At the Mn K-edge, this technique is sensitive to details of the electronic structure of the Mn atoms. We discuss the resonant x-ray spectra measured above and…

Strongly Correlated Electrons · Physics 2009-11-10 S. Grenier , J. P. Hill , Doon Gibbs , K. J. Thomas , M. v. Zimmermann , C. S. Nelson , V. Kiryukhin , Y. Tokura , D. Casa , T. Gog , C. Venkataraman

Magnetic structures and the relationship between spin and charge-orbital orderings of an A-site ordered double-perovskite manganite SmBaMn2O6, an anticipated multiferroic material, were investigated by means of neutron diffraction. The spin…

Strongly Correlated Electrons · Physics 2021-07-14 Ryoji Kiyanagi , Shigeki Yamada , Hiroshi Aoki , Hajime Sagayama , Taketo Moyoshi , Akiko Nakao , Takahisa Arima

We report the first direct resonant soft x-ray scattering observations of orbital ordering. We have studied the low temperature phase of La$_{0.5}$Sr$_{1.5}$MnO$_4$, a compound that displays charge and orbital ordering. Previous claims of…

Strongly Correlated Electrons · Physics 2009-11-10 S. B. Wilkins , P. D. Spencer , P. D. Hatton , S. P. Collins , M. D. Roper , D. Prabhakaran , A. T. Boothroyd

Resonant soft x-ray diffraction has been used to probe the temperature dependent orbital and magnetic structure of $\mathrm{LaSr_{2}Mn_{2}O_7}$. Previous crystallographic studies have shown that this material has almost no MnO$_{6}$ oxygen…

Strongly Correlated Electrons · Physics 2007-05-23 S. B. Wilkins , N. Stojic , T. A. W. Beale , N. Binggeli , P. Bencok , S. Stanescu , J. F. Mitchell , P. Abbamonte , P. D. Hatton , M. Altarelli

We present a systematic study of the electronic structure in A-site ordered manganites as function of doping and temperature. The energy dependencies observed with soft x-ray resonant diffraction (SXRD) at the Mn L_{2,3} edges are compared…

We report the study of magnetic and orbital order in Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ epitaxial thin films grown on (LaAlO$_3$)$_{0.3}$-(SrAl$_{0.5}$Ta$_{0.5}$O$_3$)$_{0.7}$ (LSAT) (011)$_c$. In a new experimental approach, the polarization and…

Strongly Correlated Electrons · Physics 2014-03-07 H. Wadati , J. Geck , E. Schierle , R. Sutarto , F. He , D. G. Hawthorn , M. Nakamura , M. Kawasaki , Y. Tokura , G. A. Sawatzky

Magnetite, Fe$_3$O$_4$, displays a highly complex low temperature crystal structure that may be charge and orbitally ordered. Many of the recent experimental claims of such ordering rely on resonant soft x-ray diffraction at the oxygen K…

Strongly Correlated Electrons · Physics 2015-05-13 S. B. Wilkins , S. Di Matteo , T. A. W. Beale , Y. Joly , C. Mazzoli , P. D. Hatton , P. Bencok , F. Yakhou , V. A. M. Brabers

Soft X-ray resonant scattering studies at the Mn $L_{\texttt{II, III}}$- and the La $M_{\texttt{IV, V}}$- edges of single-crystal LaSr$_2$Mn$_2$O$_7$ are reported. At low temperatures, below $T_\texttt{N} \approx 160$ K, energy scans with a…

Strongly Correlated Electrons · Physics 2014-07-08 H. -F. Li , Y. Su , Tapan Chatterji , A. Nefedov , J. Persson , P. Meuffels , Y. Xiao , Th. Brückel

We have investigated the low temperature phase of a Nd0.5Sr0.5MnO3 single crystal by x-ray resonant scattering at the Mn K-edge of the (3 0 0), (0 3 0) and (0 5/2 0) reflections. Strong resonances were observed for the s-s' channel in the…

Strongly Correlated Electrons · Physics 2009-11-10 Javier Herrero-Martin , Joaquin Garcia Ruiz , Gloria Subias , Javier Blasco , Maria Concepcion-Sanchez

We have studied the orbital ordering (OO) in La0.5Sr1.5MnO4 and its soft x-ray resonant diffraction spectroscopic signature at the Mn L2, L3 edges. We have modelled the system in second quantization as a small planar cluster consisting of a…

Strongly Correlated Electrons · Physics 2016-08-31 Alessandro Mirone , S. S. Dhesi , G. van der Laan

Charge and orbital ordering behaviors in the half doped bi-layered compound LaSr2Mn2O7 have been studied by resonant and non-resonant X-ray scattering. Three different order parameters, which correspond to the A-type antiferromagnetic, a…

X-ray resonant scattering at the K-edge of transition metal oxides is shown to measure the orbital order parameter, supposed to accompany magnetic ordering in some cases. Virtual transitions to the 3d-orbitals are quadrupolar in general. In…

Strongly Correlated Electrons · Physics 2009-10-30 Michele Fabrizio , Massimo Altarelli , Maurizio Benfatto

Here we show that the low temperature phase of magnetite is associated with an effective, although fractional, ordering of the charge. Evidence and a quantitative evaluation of the atomic charges are achieved by using resonant x-ray…

Strongly Correlated Electrons · Physics 2009-11-11 E. Nazarenko , J. E. Lorenzo , Y. Joly , J. L. Hodeau , D. Mannix , C. Marin

It is proposed that the observation of orbital ordering in manganite materials should be possible at the L_II and L_III edges of manganese using X-ray resonant scattering. If performed, dipole selection rules would make the measurements…

Condensed Matter · Physics 2009-10-31 C. W. M. Castleton , M. Altarelli

We present high resolution high energy and resonant x-ray diffraction results from La2-2xSr1+2xMn2O7 for x=0.55,0.575 and 0.60. These compounds show superlattice reflections at wavevectors of (h+-\delta,k+-\delta,l) and…

Strongly Correlated Electrons · Physics 2009-11-10 T. A. W. Beale , P. D. Spencer , P. D. Hatton , S. B. Wilkins , M. von Zimmermann , S. D. Brown , D. Prabhakaran , A. T. Boothroyd

Resonant x-ray diffraction performed at the $\rm L_{II}$ and $\rm L_{III}$ absorption edges of Ru has been used to investigate the magnetic and orbital ordering in Ca$_2$RuO$_4$ single crystals. A large resonant enhancement due to electric…

In a recent published paper [Phys. Rev. B 64, 195133 (2001)], Zimmermann et al. present a systematic x-ray scattering study of charge and orbital ordering phenomena in the Pr1-xCaxMnO3 series with x= 0.25, 0.4 and 0.5. They propose that for…

Strongly Correlated Electrons · Physics 2009-11-10 Joaquin Garcia , Gloria Subias

Using soft-x-ray diffraction at the site-specific resonances in the Fe L23 edge, we find clear evidence for orbital and charge ordering in magnetite below the Verwey transition. The spectra show directly that the (001/2) diffraction peak…

Strongly Correlated Electrons · Physics 2010-01-25 J. Schlappa , C. Schuessler-Langeheine , C. F. Chang , H. Ott , A. Tanaka , Z. Hu , M. W. Haverkort , E. Schierle , E. Weschke , G. Kaindl , L. H. Tjeng
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