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The semiconductor-insulator phase transition of the single-layer manganite La0.5Sr1.5MnO4 has been studied by means of high resolution synchrotron x-ray powder diffraction and resonant x-ray scattering at the Mn K edge. We conclude that a…

Strongly Correlated Electrons · Physics 2015-05-27 J. Herrero-Martin , J. Blasco , J. Garcia , G. Subias , C. Mazzoli

We performed resonant and nonresonant x-ray diffraction studies of a Nd0.5Sr0.5MnO3 thin film that exhibits a clear first-order transition. Lattice parameters vary drastically at the metal-insulator transition at 170K (=T_MI), and…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Wakabayashi , D. Bizen , H. Nakao , Y. Murakami , M. Nakamura , Y. Ogimoto , M. Izumi , K. Miyano , H. Sawa

We report on the ultrafast dynamics of charge order and structural response during the photoinduced suppression of charge and orbital order in a mixed-valence manganite. Employing femtosecond time-resolved resonant x-ray diffraction below…

Non-resonant ferromagnetic x-ray diffraction has been used to separate the spin and orbital contribution to the magnetization density of the proposed zero-moment ferromagnet $Sm_{0.982}Gd_{0.018} Al_{2}$. The alignment of the spin and…

Condensed Matter · Physics 2009-11-07 J. W. Taylor , J. A. Duffy , A. M. Bebb , M. R. Lees , L. Bouchenoire , S. D. Brown , M. J. Cooper

The high-pressure synthesized quasi-one-dimensional compounds NaMn$_2$O$_4$ and Li$_{0.92}$Mn$_2$O$_4$ are both antiferromagnetic insulators, and here their atomic and magnetic structures were investigated using neutron powder diffraction.…

Antiferroquadrupolar (AFQ) ordering has been conjectured in several rare-earth compounds to explain their anomalous magnetic properties. No direct evidences for AFQ ordering, however, have been reported. Using the resonant x-ray scattering…

Strongly Correlated Electrons · Physics 2009-10-31 K. Hirota , N. Oumi , T. Matsumura , H. Nakao , Y. Wakabayashi , Y. Murakami , Y. Endoh

The magnetic ordering of the hexagonal multiferroic compound YbMnO$_3$ has been studied between 100 K and 1.5 K by combining neutron powder diffraction, $^{170}$Yb M\"ossbauer spectroscopy and magnetization measurements. The Yb moments of…

Strongly Correlated Electrons · Physics 2008-09-30 X. Fabrèges , I. Mirebeau , P. Bonville , S. Petit , G. Lebras-Jasmin , A. Forget , G. André , S. Pailhès

Resonant x-ray scattering is performed near the Mn K-absorption edge for an epitaxial thin film of BiMnO3. The azimuthal angle dependence of the resonant (003) peak (in monoclinic indices) is measured with different photon polarizations;…

Materials Science · Physics 2009-11-11 C. -H. Yang , J. Koo , C. Song , T. Y. Koo , K. -B. Lee , Y. H. Jeong

We have studied the magnetic ordering in Na doped BaFe$_2$As$_2$ by unpolarized and polarized neutron diffraction using single crystals. Unlike previously studied FeAs-based compounds that magnetically order, Ba$_{1-x}$Na$_x$Fe$_2$As$_2$…

Superconductivity · Physics 2015-06-22 F. Wasser , A. Schneidewind , Y. Sidis , S. Aswartham , S. Wurmehl , B. Buchner , M. Braden

We use resonant X-ray scattering at the nickel L$_{2,3}$ edges to investigate the interplay between orbital degrees of freedom and charge density waves (CDW) in the superconductor BaNi$_2$(As$_{1-x}$P$_x$)$_2$. Both the incommensurate and…

A single crystal of GdBaCo2O5.47(2) has been studied by means of X-ray diffraction. Appearance of superstructure reflections at T = 341.5(7) K gives an evidence of continuous transition to the phase with unit cell doubled along the shortest…

Materials Science · Physics 2009-11-10 Yu. P. Chernenkov , V. P. Plakhty , V. I. Fedorov , S. N. Barilo , S. V. Shiryaev , G. L. Bychkov

The crystallographic and magnetic phase diagram of the n=2 layered manganite La2-2xSr1+2xMn2O7 in the region x=>0.5 has been studied using temperature dependent neutron powder diffraction. The magnetic phase diagram reveals a progression of…

Materials Science · Physics 2009-10-31 C. D. Ling , J. E. Millburn , J. F. Mitchell , D. N. Argyriou J. Linton , H. N. Bordallo

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low…

Strongly Correlated Electrons · Physics 2016-11-24 S. M. Souliou , Y. Li , X. Du , M. Le Tacon , A. Bosak

We present diffraction data on a single-layered manganite La(0.42)Sr(1.58)MnO4 with hole doping (x>0.5). Overdoped La(0.42)Sr(1.58)MnO4 exhibits a complex ordering of charges, orbitals and spins. Single crystal neutron diffraction…

Strongly Correlated Electrons · Physics 2012-01-12 H. Ulbrich , D. Senff , P. Steffens , O. J. Schumann , Y. Sidis , P. Reutler , A. Revcolevschi , M. Braden

In a recent letter, E. Nazarenko et al [Phys. Rev. Lett. 97, 056403 (2006) and cond-mat/0606596] have investigated the low temperature phase of magnetite by means of resonant X-ray scattering. The paper puts forward the quantitative…

Strongly Correlated Electrons · Physics 2008-02-05 Joaquin Garcia , Gloria Subias , Javier Blasco , Ma Grazia Proietti , Hubert Renevier

The electronic structure of the doped manganites Pr$_{1-x}$Ca$_x$MnO$_3$ was calculated by the LSDA+U method which takes into account the local Coulomb interaction between d-electrons of transition metal ions. In contrast to the standard…

Condensed Matter · Physics 2009-10-28 V. I. Anisimov , I. S. Elfimov , M. A. Korotin , K. Terakura

The weakly interacting S=1/2 dimers system Sr3Cr2O8 has been investigated by powder neutron diffraction and inelastic neutron scattering. Our data reveal a structural phase transition below room temperature corresponding to an…

Materials Science · Physics 2008-07-10 L. C. Chapon , C. Stock , P. G. Radaelli , C. Martin

Neutron diffraction, polarized neutron transmission, and small angle neutron scattering have been used to investigate the crystal structure and nature of the magnetic order in a polycrystalline sample of RuSr2Eu1.2Ce0.8Cu2O10. The sample…

Superconductivity · Physics 2009-11-11 J. W. Lynn , Y. Chen , Q. Huang , S. K. Goh , G. V. M. Williams , J. L. Tallon

Through powder x-ray diffraction we have investigated the structural behavior of SmVO3, in which orbital and magnetic degrees of freedom are believed to be closely coupled to the crystal lattice. We have found, contrary to previous reports,…

The temperature dependence of the electron-spin resonance linewidth in La0.95Sr0.05MnO3 has been determined and analyzed in the paramagnetic regime across the orbital ordering transition. From the temperature dependence and the anisotropy…

Strongly Correlated Electrons · Physics 2009-11-10 J. Deisenhofer , B. I. Kochelaev , E. Shilova , A. M. Balbashov , A. Loidl , H. -A. Krug von Nidda