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Propylene carbonate (PC) wets graphite with a contact angle of 31 deg at ambient conditions. Molecular dynamics simulations agree with this contact angle after 40% reduction of the strength of graphite-C atom Lennard-Jones interactions with…

We employ molecular dynamic simulations to study the reduction process of graphene-oxide (GO) in a chemically active environment enriched with hydrogen. We examine the concentration and pressure of hydrogen gas as a function of temperature…

Materials Science · Physics 2016-09-28 Ramin M. Abolfath , Kyeongjae Cho

This paper presents an experimental and modeling study of the oxidation of large linear akanes (from C10) representative from diesel fuel from low to intermediate temperature (550-1100 K) including the negative temperature coefficient (NTC)…

Distributed combustion, often associated with the low-oxygen condition, offers ultra-low NOX emission. However, it was recently achieved without combustion air dilution or internal flue gas recirculation, using a distinct approach called…

Fluid Dynamics · Physics 2022-04-20 Dániel Füzesi , Milan Malý , Jan Jedelský , Viktor Józsa

We show that converging spherical and cylindrical shock waves may ignite a detonation wave in a combustible medium, provided the radius at which the shocks become strong exceeds a critical radius, R_c. An approximate analytic expression for…

High Energy Astrophysical Phenomena · Physics 2015-05-30 Doron Kushnir , Eli Livne , Eli Waxman

A minimal model for curved detonations is studied, illustrating the role of the reaction rate on the detonation speed and its propagation limits. The model is based on a simple extension of the minimal Fickett toy model for detonations…

Fluid Dynamics · Physics 2023-12-08 Matei Ioan Petru Rădulescu , Aliou Sow

This work reports a theoretical study of the gas phase unimolecular decomposition of cyclobutane, cyclopentane and cyclohexane by means of quantum chemical calculations. A biradical mechanism has been envisaged for each cycloalkane, and the…

Chemical Physics · Physics 2009-04-28 Baptiste Sirjean , Pierre-Alexandre Glaude , M. F. Ruiz-Lopez , René Fournet

In this paper we consider ignition-temperature, first-order reaction model of thermo-diffusive combustion that describes dynamics of thick flames arising in a theory of combustion of hydrogen-oxygen and ethylene-oxygen mixtures. These…

Chaotic Dynamics · Physics 2017-04-03 Nathan Kilker , Dmitry Golovaty , Peter V. Gordon , Leonid Kagan , Gregory I. Sivashinsky

We study water-hydrogen mixtures under planetary interior conditions using ab initio molecular dynamics simulations. We determine the thermodynamic properties of various water-hydrogen mixing ratios at temperatures of 2000 and 6000 K for…

Earth and Planetary Astrophysics · Physics 2015-10-28 Francois Soubiran , Burkhard Militzer

The problem of detonation attenuation in stoichiometric methane-oxygen and its re-establishment following its interaction with obstacles was investigated using high resolution numerical simulation. The main focus was on the role of the…

Fluid Dynamics · Physics 2022-11-02 Grace Floring , Mohnish Peswani , Brian Maxwell

Biofuels have shown to be a reliable source of energy and a replication of fossil fuels. A well-known branch of biofuels is oxygenated ones derived from lignin compounds. Although a wide range of studies was done on oxygenated fuels,…

Fluid Dynamics · Physics 2018-06-20 Saeid Zare , Lameed Ayo Onigbanjo , Shrabanti Roy , Omid Askari

In contrast to carbon, which forms long polymeric chains, all-nitrogen chains are very unstable. Here we found that nitrogen and hydrogen directly react at room temperature and pressures of about 35 GPa forming a mixture of nitrogen…

Materials Science · Physics 2014-09-09 H. Wang , M. I. Eremets , I. Troyan , H. Liu , Y. Ma , L. Vereecken

We show experimentally and numerically that when a weak shock interacts with a finger flame in a narrow channel, an extremely efficient mechanism for deflagration to detonation transition occurs. This is demonstrated in a 19-mm-thick…

Fluid Dynamics · Physics 2019-11-14 Hongxia Yang , Matei I. Radulescu

PDF model calculations have been performed of the Cabra lifted hydrogen flame in a vitiated co-flow. Particle trajectories are extracted from the Lagrangian particle method used to solve the modeled PDF equation. The particle trajectories…

Fluid Dynamics · Physics 2007-09-10 Haifeng Wang , Stephen B. Pope

Hydrogen adsorption by graphite is examined by classical molecular dynamics simulation using a modified Brenner REBO potential. Such interactions are typical in chemical sputtering experiments, and knowledge of the fundamental behavior of…

Soft Condensed Matter · Physics 2009-11-11 A. Ito , H. Nakamura

Premixed flames propagating within small channels show complex combustion phenomena that differ from flame propagation at conventional scales. Available experimental and numerical studies have documented stationary/non-stationary and/or…

Fluid Dynamics · Physics 2016-08-02 Mohsen Ayoobi , Ingmar Schoegl

The detonation behaviors during thermonuclear burning indicate a state of robust hot spot burning and are widely present in astronomical phenomena, such as supernovae. In this work, we propose an analytical model including alpha-particle…

Plasma Physics · Physics 2024-12-18 Bohan Shen , Junjue Liao , Renjie He , Zekun Xu , Fuyuan Wu , Jie Zhang

Few-layer graphene (FLG) is grown on copper and nickel substrates at high rates using a novel flame synthesis method in open-atmosphere environments. Transmittance and resistance properties of the transferred films are similar to those…

The mechanisms of direct detonation initiation (DDI) in methane/air mixtures containing coal particles are investigated through simulations conducted using the Eulerian-Lagrangian method in a two-dimensional configuration. Methane-air…

Chemical Physics · Physics 2025-03-05 Shengnan Li , Shangpeng Li , Shumeng Xie , Yong Xu , Ke Gao , Huangwei Zhang

Theory and computations have established that thermodynamic gradients created by hot spots in reactive gas mixtures can lead to spontaneous detonation initiation. However, the current laminar theory of the temperature-gradient mechanism for…

Fluid Dynamics · Physics 2019-11-26 Colin A. Z. Towery , Alexei Y. Poludnenko , Peter E. Hamlington
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