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Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

Materials Science · Physics 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

We use above-bandgap optical excitation, via a 1047 nm laser, to hyperpolarize the $^{31}$P spins in low-doped (N$_D =6\times10^{15}$ cm$^{-3}$) natural abundance silicon at 4.2 K and 6.7 T, and inductively detect the resulting NMR signal.…

Mesoscale and Nanoscale Physics · Physics 2018-11-21 P. Gumann , H. Haas , S. Sheldon , L. Zhu , M. L. W. Thewalt , D. G. Cory , C. Ramanathan

Hyper-polarization of nuclear spins is crucial for advancing nuclear magnetic resonance (NMR) and quantum information technologies, as nuclear spins typically exhibit extremely low polarization at room temperature due to their small…

Quantum Physics · Physics 2025-05-20 Haiyang Li , Hao Liao , Ping Wang

We propose schemes to produce highly nuclear-spin polarized small molecules in an intense and cold molecular beam via microwave or infrared rotational excitation, followed by hyperfine-induced quantum beats. Repumping schemes can be used to…

Chemical Physics · Physics 2026-03-20 C. S. Kannis , T. P. Rakitzis

As the deepest group V donor in Si, Bi has by far the largest hyperfine interaction, and also a large I=9/2 nuclear spin. At zero field this splits the donor ground state into states having total spin 5 and 4, which are fully resolved in…

Quantum Physics · Physics 2010-06-03 T. Sekiguchi , M. Steger , K. Saeedi , M. L. W. Thewalt , H. Riemann , N. V. Abrosimov , N. Noetzel

Nuclear spin polarization induced by hyperfine interaction and the Edelstein effect due to strong spin-orbit interaction is investigated by quantum transport in Bi(111) thin film samples. The Bi(111) films are deposited on mica by van der…

Mesoscale and Nanoscale Physics · Physics 2020-09-09 Zijian Jiang , Victoria Soghomonian , Jean J. Heremans

Magnetic resonance imaging in ultra-low fields is often limited by mediocre signal-to-noise ratio hindering a higher resolution. Overhauser dynamic nuclear polarisation (O-DNP) using nitroxide radicals has been an efficient solution for…

We propose an approach to probe coherent spin-state dynamics of molecules using circularly polarized hard x-ray pulses. For the dynamically aligned nitric oxide molecules in a coherent superposition spin-orbit coupled electronic state that…

Optics · Physics 2024-01-02 Xiaoyu Mi , Ming Zhang , Zheng Li

Relaxation of conduction electron spins in a semiconductor owing to the hyperfine interaction with spin-1/2 nuclei, in zero applied magnetic field, is investigated. We calculate the electron spin relaxation time scales, in order to evaluate…

Mesoscale and Nanoscale Physics · Physics 2010-10-12 Yuriy V. Pershin , Vladimir Privman

Nuclear spin hyperpolarization provides a promising route to overcome the challenges imposed by the limited sensitivity of nuclear magnetic resonance. Here we demonstrate that dissolution of spin-polarized pentacene-doped naphthalene…

We polarize nuclear spins in a GaAs double quantum dot by controlling two-electron spin states near the anti-crossing of the singlet (S) and m_S=+1 triplet (T+) using pulsed gates. An initialized S state is cyclically brought into resonance…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. R. Petta , J. M. Taylor , A. C. Johnson , A. Yacoby , M. D. Lukin , C. M. Marcus , M. P. Hanson , A. C. Gossard

Color-center-hosting semiconductors are emerging as promising source materials for low-field dynamic nuclear polarization (DNP) at or near room temperature, but hyperfine broadening, susceptibility to magnetic field heterogeneity, and…

Quantum Physics · Physics 2022-06-01 J. Henshaw , D. Pagliero , P. R. Zangara , B. Franzoni , A. Ajoy , R. Acosta , J. A. Reimer , A. Pines , C. A. Meriles

We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

The role of staggered potential on light-induced spin and pseudo-spin polarization has been investigated in silicene. It has been shown that non-equilibrium spin and pseudo-spin polarizations are emerged in silicene sheet by applying an…

Mesoscale and Nanoscale Physics · Physics 2020-05-25 N. Shahabi , A. Phirouznia

In a dynamic nuclear polarization experiment on a 40 mM solution of 4-amino-TEMPO in a 40:60 water/glycerol mixture, we have observed that the bulk dipolar reservoir is cooled to a spin temperature of 15.5 micro-K, following microwave…

Other Condensed Matter · Physics 2009-04-01 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

Photochemically induced dynamic nuclear polarization (photo-CIDNP) is a method to hyperpolarize nuclear spins using light. In most cases, CIDNP experiments are performed at a high magnetic field and the sample is irradiated by the light…

A large $\mu^-$ polarization was achieved in muonic Bi atoms with the help of the strong hyperfine field in a polarized nuclear target. Using $^{209}$Bi nuclei polarized to ($59\pm9$)% in ferromagnetic BiMn, we observed a $\mu$-$e$ decay…

A quasi-classical theoretical description of polarization and relaxation of nuclear spins in a quantum dot with one resident electron is developed for arbitrary mechanisms of electron spin polarization. The dependence of the…

Strongly Correlated Electrons · Physics 2015-05-13 I. A. Merkulov , G. Alvarez , D. R. Yakovlev , T. C. Schulthess

The nuclear spin state of a phosphorus donor ($^{31}$P) in isotopically enriched silicon-28 is an excellent host to store quantum information in the solid state. The spin's insensitivity to electric fields yields a solid-state qubit with…

Mesoscale and Nanoscale Physics · Physics 2018-09-12 Guilherme Tosi , Fahd A. Mohiyaddin , Stefanie Tenberg , Arne Laucht , Andrea Morello

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin
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