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We present an experimental study of the dynamics underlying the buildup and decay of dynamical nuclear spin polarization in a single semiconductor quantum dot. Our experiment shows that the nuclei can be polarized on a time scale of a few…

Optics · Physics 2007-08-02 P. Maletinsky , A. Badolato , A. Imamoglu

Dynamic nuclear polarization (DNP) is capable of boosting signals in nuclear magnetic resonance by orders of magnitude by creating out-of-equilibrium nuclear spin polarization. The diffusion of nuclear spin polarization in the vicinity of…

Other Condensed Matter · Physics 2023-07-12 Alessandro Chessari , Samuel F. Cousin , Sami Jannin , Quentin Stern

The nuclear polarization of $\mathrm{H}_2$ molecules formed by recombination of nuclear polarized H atoms on the surface of a storage cell initially coated with a silicon-based polymer has been measured by using the longitudinal double-spin…

Atomic Physics · Physics 2012-08-27 The HERMES collaboration

There has been much renewed interest in dynamic nuclear polarization (DNP), particularly in the context of solid state biomolecular NMR and more recently dissolution DNP techniques for liquids. This paper reviews the role of spin diffusion…

Other Condensed Matter · Physics 2009-04-01 Chandrasekhar Ramanathan

The ground state of an acceptor-bound hole in a zinc-blende semiconductor is formed by four eigenstates of the total angular momentum, which is a vector sum of spin and orbital moment of the hole. As a result, the hyperfine interaction of…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 K. V. Kavokin , A. V. Koudinov

Silicon carbide (SiC)-based defects are promising for quantum communications, quantum information processing, and for the next generation of quantum sensors, as they feature long coherence times, frequencies near the telecom, and optical…

Quantum Physics · Physics 2019-05-15 Wenzheng Dong , M. W. Doherty , Sophia E. Economou

Spin polarized states in nuclear matter with an effective nucleon-nucleon interaction are studied for a wide range of isospin asymmetries and densities. Based on a Fermi liquid theory, it is shown that there are a few possible scenarios of…

Nuclear Theory · Physics 2007-09-22 A. A. Isayev

Silicon-based qubits are often made by trapping individual electrons in quantum dots defined by electric gates. Quantum information can then be stored using the spin states of the electrons. However, the nuclei of the surrounding atoms also…

Mesoscale and Nanoscale Physics · Physics 2025-05-09 Xinxin Cai , Habitamu Y. Walelign , John M. Nichol

Spontaneous nuclear polarization is predicted in double quantum dots in the spin-blocked electron transport regime. The polarization results from an instability of the zero-polarization state when singlet and triplet electron energy levels…

Mesoscale and Nanoscale Physics · Physics 2010-08-23 M. S. Rudner , L. S. Levitov

Spatially nonhomogeneously spin polarized nuclei are proposed as a new mechanism to monitor electron states in a nanostructure, or as a means to createn and, if necessary, reshape such nanostructures in the course of the experiment. We…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 V. Fleurov , V. A. Ivanov , F. M. Peeters , I. D. Vagner

Intermediate-energy heavy-ion collisions can produce a spin polarization of the projectile-like species. Spin polarization has been observed for both nucleon removal and nucleon pickup processes. Qualitative agreement with measured spin…

Nuclear Experiment · Physics 2008-11-26 D. E. Groh , J. S. Pinter , P. F. Mantica , T. J. Mertzimekis , A. E. Stuchbery , D. T. Khoa

We report on the dynamic nuclear polarization of a single charge-tunable self-assembled InAs/GaAs quantum dot in a longitudinal magnetic field of $\sim$0.2T. The hyperfine interaction between the optically oriented electron and nuclei spins…

Dynamic nuclear polarization experiments use microwave irradiation to transfer the larger electron polarization to nuclear spins of interest, and thus enhance the NMR transitions above thermal equilibrium. How the polarization transfer from…

Chemical Physics · Physics 2026-01-12 Gian-Marco Camenisch , Nino Wili , Gunnar Jeschke , Matthias Ernst

Dynamical nuclear polarisation (DNP) is an important technique that uses polarisation transfer from electron to nuclear spins to achieve nuclear hyperpolarisation. As the electron spin of the nitrogen vacancy (NV) centres in diamond can be…

A new method for local dynamic nuclear polarization is demonstrated in a GaAs/AlGaAs heterostructure at the Landau level filling factor $\nu=3$. Using a narrow channel sample, where the width varies stepwise along the electron flow, we find…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yosuke Komori , Tohru Okamoto

In dissolution-dynamic nuclear polarization, nuclear spins are hyperpolarized at cryogenic temperatures using radicals and microwave irradiation. The hyperpolarized solid is dissolved with hot solvent and the solution is transferred to a…

Instrumentation and Detectors · Physics 2019-06-20 Karel Kouřil , Hana Kouřilová , Samuel Bartram , Malcolm H. Levitt , Benno Meier

We studied the dynamic nuclear spin polarization of nitrogen in negatively charged nitrogen-vacancy (NV) centers in diamond both experimentally and theoretically over a wide range of magnetic fields from 0 to 1100 G covering both the…

Quantum Physics · Physics 2021-01-04 Laima Busaite , Reinis Lazda , Andris Berzins , Marcis Auzinsh , Ruvin Ferber , Florian Gahbauer

Understanding fully the dynamics of coupled electron-nuclear spin systems, which are important for the development of long-lived qubits based on solid-state systems, remains a challenge. We show that in a singly charged semiconductor…

Mesoscale and Nanoscale Physics · Physics 2010-07-26 Wenxian Zhang , Jian-Liang Hu , Jun Zhuang , J. Q. You , Ren-Bao Liu

Dynamic nuclear polarization (DNP) has revolutionized the field of NMR spectroscopy, expanding its reach and capabilities to investigate diverse materials, biomolecules, and complex dynamic processes. Bringing high-efficiency DNP to the…

Mesoscale and Nanoscale Physics · Physics 2024-02-27 Sahand Tabatabaei , Pritam Priyadarsi , Namanish Singh , Pardis Sahafi , Daniel Tay , Andrew Jordan , Raffi Budakian

In dynamic nuclear polarization (DNP) experiments, the compound is driven out-of-equilibrium by microwave (MW) irradiation of the radical electron spins. Their stationary state has been recently probed via electron double resonance (ELDOR)…

Strongly Correlated Electrons · Physics 2017-02-28 Filippo Caracciolo , Marta Filibian , Pietro Carretta , Alberto Rosso , Andrea De Luca