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X-ray spectroscopy of rare-earth nickelate LuNiO$_3$: LDA+DMFT study

Strongly Correlated Electrons 2020-09-09 v1 Materials Science

Abstract

We present a computational study of resonant inelastic x-ray scattering (RIXS) and x-ray absorption in a representative rare-earth nickelate LuNiO3_3. We study the changes in the spectra across the metal-insulator/site-disproportionation transition. In particular, we address the question of site-selectivity of the two methods in the disproportionated insulating phase and the signature of metal-insulator transition in the fluorescence-like feature of the RIXS spectra. To this end we use the local density approximation + dynamical mean-field theory (LDA+DMFT) approach combined with configuration integration method to compute the core-level spectra.

Keywords

Cite

@article{arxiv.2004.01428,
  title  = {X-ray spectroscopy of rare-earth nickelate LuNiO$_3$: LDA+DMFT study},
  author = {Mathias Winder and Atsushi Hariki and Jan Kuneš},
  journal= {arXiv preprint arXiv:2004.01428},
  year   = {2020}
}