Low-valence nickelates − including infinite-layer (IL) and trilayer (TL) compounds − are longstanding candidates for mimicking the high-temperature superconductivity of cuprates. A recent breakthrough in the field came with the discovery of superconductivity in hole-doped IL nickelates. Yet, the degree of similarity between low-valence nickelates and cuprates is the subject of a profound debate for which soft x-ray spectroscopy experiments at the Ni L- and O K-edge provided critical input. In this review, we will discuss the essential elements of the electronic structure of low-valance nickelates revealed by x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS). Furthermore, we will review magnetic excitations observed in the RIXS spectra of IL and TL nickelates, which exhibit characteristics that are partly reminiscent of those of cuprates.
@article{arxiv.2111.02511,
title = {Soft X-ray Spectroscopy of Low-Valence Nickelates},
author = {M. Hepting and M. P. M. Dean and W. S. Lee},
journal= {arXiv preprint arXiv:2111.02511},
year = {2022}
}
Comments
11 pages, 2 figures, submitted to the Condensed Matter Physics section in Frontiers in Physics for the research topic "Advances in Superconducting Infinite-Layer and Related Nickelates"