English

Writing and detecting topological charges in exfoliated Fe$_{5-x}$GeTe$_2$

Mesoscale and Nanoscale Physics 2024-01-17 v1

Abstract

Fe5x_{5-x}GeTe2_2 is a promising two-dimensional (2D) van der Waals (vdW) magnet for practical applications, given its magnetic properties. These include Curie temperatures above room temperature, and topological spin textures (TST or both merons and skyrmions), responsible for a pronounced anomalous Hall effect (AHE) and its topological counterpart (THE), which can be harvested for spintronics. Here, we show that both the AHE and THE can be amplified considerably by just adjusting the thickness of exfoliated Fe5x_{5-x}GeTe2_2, with THE becoming observable even in zero magnetic field due to a field-induced unbalance in topological charges. Using a complementary suite of techniques, including electronic transport, Lorentz transmission electron microscopy, and micromagnetic simulations, we reveal the emergence of substantial coercive fields upon exfoliation, which are absent in the bulk, implying thickness-dependent magnetic interactions that affect the TST. We detected a ``magic" thickness tt \sim 30 nm where the formation of TST is maximized, inducing large magnitudes for the topological charge density (6.45×10206.45 \times 10^{20} cm2^{-2}), and the concomitant anomalous (ρxyA,max22.6\rho_{xy}^{\text{A,max}} \simeq 22.6 μΩ\mu \Omega cm) and topological (ρxyu,T15\rho_{xy}^{\text{u,T}} \simeq 15 μΩ\mu \Omega cm) Hall resistivities at TT ~ 120 K. These values for ρxyA,max\rho_{xy}^{\text{A,max}} and ρxyu,T\rho_{xy}^{\text{u,T}} are higher than those found in magnetic topological insulators and, so far, the largest reported for 2D magnets. The hitherto unobserved THE under zero magnetic field could provide a platform for the writing and electrical detection of TST aiming at energy-efficient devices based on vdW ferromagnets.

Keywords

Cite

@article{arxiv.2401.07156,
  title  = {Writing and detecting topological charges in exfoliated Fe$_{5-x}$GeTe$_2$},
  author = {Alex Moon and Yue Li and Conor McKeever and Brian W. Casas and Moises Bravo and Wenkai Zheng and Juan Macy and Amanda K. Petford-Long and Gregory T. McCandless and Julia Y. Chan and Charudatta Phatak and Elton J. G. Santos and Luis Balicas},
  journal= {arXiv preprint arXiv:2401.07156},
  year   = {2024}
}

Comments

45 pages with supporting information file, 5 main figures. Accepted ACS Nano 2024