English

Large anomalous Hall effect in layered antiferromagnet Co$_{0.29}$TaS$_2$

Materials Science 2022-03-25 v1

Abstract

We present a study on the magnetization, anomalous Hall effect (AHE) and novel longitudinal resistivity in layered antiferromagnet Co0.29_{0.29}TaS2_{2}. Of particular interests in Co0.29_{0.29}TaS2_{2} are abundant magnetic transitions, which show that the magnetic structures are tuned by temperature or magnetic field. With decreasing temperature, Co0.29_{0.29}TaS2_{2} undergoes two transitions at Tt1_{t1}\sim 38.3 K and Tt2_{t2}\sim 24.3 K. Once the magnetic field is applied, another transition Tt3_{t3}\sim 34.3 K appears between 0.3 T and 5 T. At 2 K, an obvious ferromagnetic hysteresis loop within Ht1±_{t1}\sim\pm 6.9 T is observed, which decreases with increasing temperature and eventually disappears at Tt2_{t2}. Besides, Co0.29_{0.29}TaS2_{2} displays step-like behavior as another magnetic transition around Ht2±_{t2}\sim\pm 4 T, which exists until \sim Tt1_{t1}. These characteristic temperatures and magnetic fields mark complex magnetic phase transitions in Co0.29_{0.29}TaS2_{2}, which are also evidenced in transport results. Large AHE dominates in the Hall resistivity with the conspicuous value of Rs_{s}/R0105_{0}\sim 10^{5}, considering that the tiny net magnetization (0.0094μB\mu_{B}/Co) alone would not lead to this value, thus the contribution of Berry curvature is necessary. The longitudinal resistivity illustrates a prominent irreversible behavior within Ht1_{t1}. The abrupt change at Ht2_{t2} below Tt1_{t1}, corresponding to the step-like magnetic transitions, is also observed. Synergy between the magnetism and topological properties, both playing a crucial role, may be the key factor of large AHE in antiferromagnet, which also offers a new perspective in magnetic topological materials with the platform of Co0.29_{0.29}TaS2_{2}.

Keywords

Cite

@article{arxiv.2203.12771,
  title  = {Large anomalous Hall effect in layered antiferromagnet Co$_{0.29}$TaS$_2$},
  author = {Huan Wang and Jun-Fa Lin and Xiang-Yu Zeng and Xiao-Ping Ma and Jing Gong and Zheng-Yi Dai and Xiao-Yan Wang and Kun Han and Yi-Ting Wang and Tian-Long Xia},
  journal= {arXiv preprint arXiv:2203.12771},
  year   = {2022}
}

Comments

5 pages,4 figures