We report ferromagnetism in 2H-Co0.22TaS2 single crystals where Co atoms are intercalated in the van der Waals gap, and a systematic study of its magnetic critical behavior in the vicinity of Tc∼28 K. The obtained critical exponents β = 0.43(2), γ = 1.15(1), and δ=3.54(1) fulfill the Widom scaling relation δ=1+γ/β and follow the scaling equation. This indicates that the spin coupling in 2H-Co0.22TaS2 is of three-dimensional Hersenberg type coupled with long-range magnetic interaction, and that the exchange interaction decays with distance as J(r)≈r−4.69. 2H-Co0.22TaS2 exhibits a weak temperature-dependent metallic behavior in resistivity and negative values of thermopower with dominant electron-type carriers, in which obvious anomalies were observed below Tc as well as the anomalous Hall effect (AHE). The linear scaling behavior between the modified anomalous Hall resistivity ρxy/μ0H and longitudinal resistivity ρxx2M/μ0H implies that the origin of AHE in 2H-Co0.22TaS2 should be dominated by the extrinsic side-jump mechanism.
@article{arxiv.2110.11350,
title = {Magnetic critical behavior and anomalous Hall effect in 2H-Co$_{0.22}$TaS$_{2}$ single crystals},
author = {Yu Liu and Zhixiang Hu and Eli Stavitski and Klaus Attenkofer and C. Petrovic},
journal= {arXiv preprint arXiv:2110.11350},
year = {2021}
}
Comments
arXiv admin note: text overlap with arXiv:2110.10908