English

Magnetic critical behavior and anomalous Hall effect in 2H-Co$_{0.22}$TaS$_{2}$ single crystals

Materials Science 2021-10-25 v1

Abstract

We report ferromagnetism in 2H-Co0.22_{0.22}TaS2_2 single crystals where Co atoms are intercalated in the van der Waals gap, and a systematic study of its magnetic critical behavior in the vicinity of Tc28T_c \sim 28 K. The obtained critical exponents β\beta = 0.43(2), γ\gamma = 1.15(1), and δ=3.54(1)\delta = 3.54(1) fulfill the Widom scaling relation δ=1+γ/β\delta = 1+\gamma/\beta and follow the scaling equation. This indicates that the spin coupling in 2H-Co0.22_{0.22}TaS2_2 is of three-dimensional Hersenberg type coupled with long-range magnetic interaction, and that the exchange interaction decays with distance as J(r)r4.69J(r)\approx r^{-4.69}. 2H-Co0.22_{0.22}TaS2_2 exhibits a weak temperature-dependent metallic behavior in resistivity and negative values of thermopower with dominant electron-type carriers, in which obvious anomalies were observed below TcT_c as well as the anomalous Hall effect (AHE). The linear scaling behavior between the modified anomalous Hall resistivity ρxy/μ0H\rho_{xy}/\mu_0H and longitudinal resistivity ρxx2M/μ0H\rho_{xx}^2M/\mu_0H implies that the origin of AHE in 2H-Co0.22_{0.22}TaS2_2 should be dominated by the extrinsic side-jump mechanism.

Keywords

Cite

@article{arxiv.2110.11350,
  title  = {Magnetic critical behavior and anomalous Hall effect in 2H-Co$_{0.22}$TaS$_{2}$ single crystals},
  author = {Yu Liu and Zhixiang Hu and Eli Stavitski and Klaus Attenkofer and C. Petrovic},
  journal= {arXiv preprint arXiv:2110.11350},
  year   = {2021}
}

Comments

arXiv admin note: text overlap with arXiv:2110.10908