English

Universal sublinear resistivity in vanadium kagome materials hosting charge density waves

Strongly Correlated Electrons 2024-07-16 v2

Abstract

The recent discovery of a charge density (CDW) state in ScV6_6Sn6_6 at TCDWT_{\textrm{CDW}} = 91 K offers new opportunities to understand the origins of electronic instabilities in topological kagome systems. By comparing to the isostructural non-CDW compound LuV6_6Sn6_6, we unravel interesting electrical transport properties in ScV6_6Sn6_6, above and below the charge ordering temperature. We observed that by applying a magnetic field along the aa axis, the temperature behavior of the longitudinal resistivity in ScV6_6Sn6_6 changes from metal-like to insulator-like above the CDW transition. We show that in the charge ordered state ScV6_6Sn6_6 follows the Fermi liquid behavior while above that, it transforms into a non-Fermi liquid phase in which the resistivity varies sublinearly over a broad temperature range. The sublinear resistivity, which scales by T3/5T^{3/5} is a common feature among other vanadium-containing kagome compounds exhibiting CDW states such as KV3_3Sb5_5, RbV3_3Sb5_5, and CsV3_3Sb5_5. By contrast, the non-Fermi liquid behavior does not occur in LuV6_6Sn6_6. We explain the T3/5T^{3/5} universal scaling behavior from the Coulomb scattering between Dirac electrons and Van Hove singularities; common features in the electronic structure of kagome materials. Finally, we show anomalous Hall-like behavior in ScV6_6Sn6_6 below TCDWT_{\textrm{CDW}}, which is absent in the Lu compound. Comparing the transport properties of ScV6_6Sn6_6 and LuV6_6Sn6_6 is valuable to highlight the impacts of the unusual CDW in the Sc compound.

Keywords

Cite

@article{arxiv.2305.02393,
  title  = {Universal sublinear resistivity in vanadium kagome materials hosting charge density waves},
  author = {Shirin Mozaffari and William R. Meier and Richa P. Madhogaria and Nikolai Peshcherenko and Seoung-Hun Kang and John W. Villanova and Hasitha W. Suriya Arachchige and Guoxin Zheng and Yuan Zhu and Kuan-Wen Chen and Kaila Jenkins and Dechen Zhang and Aaron Chan and Lu Li and Mina Yoon and Yang Zhang and David G. Mandrus},
  journal= {arXiv preprint arXiv:2305.02393},
  year   = {2024}
}

Comments

12 pages, 6 figures. Power law behavior of resistivity as a function temperature is modified and theoretical explanation is added in the second version

R2 v1 2026-06-28T10:24:59.775Z