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Superconductivity emerging from density-wave-like order in a correlated kagome metal

Superconductivity 2024-09-04 v2 Materials Science Strongly Correlated Electrons

Abstract

Unconventional superconductivity (USC) in a highly correlated kagome system has been theoretically proposed for years, yet the experimental realization is hard to achieve. The recently discovered vanadium-based kagome materials, which exhibit both superconductivity and charge density wave (CDW) orders, are nonmagnetic and weakly correlated, thus unlikely host USC as theories proposed. Here we report the discovery of a chromium-based kagome metal, CsCr3_3Sb5_5, which is contrastingly characterised by strong electron correlations, frustrated magnetism, and characteristic flat bands close to the Fermi level. Under ambient pressure, it undergoes a concurrent structural and magnetic phase transition at 55 K, accompanying with a stripe-like 4a04a_0 structural modulation. At high pressure, the phase transition evolves into two transitions, probably associated with CDW and antiferromagnetic spin-density-wave orderings, respectively. These density-wave (DW)-like orders are gradually suppressed with pressure and, remarkably, a superconducting dome emerges at 3.65-8.0 GPa. The maximum of the superconducting transition temperature, Tcmax=T_\mathrm{c}^{\mathrm{max}}= 6.4 K, appears when the DW-like orders are completely suppressed at 4.2 GPa, and the normal state exhibits a non-Fermi-liquid behaviour, reminiscent of USC and quantum criticality in iron-based superconductors. Our work offers an unprecedented platform for investigating possible USC in a correlated kagome system.

Keywords

Cite

@article{arxiv.2309.13514,
  title  = {Superconductivity emerging from density-wave-like order in a correlated kagome metal},
  author = {Yi Liu and Zi-Yi Liu and Jin-Ke Bao and Peng-Tao Yang and Liang-Wen Ji and Si-Qi Wu and Qin-Xin Shen and Jun Luo and Jie Yang and Ji-Yong Liu and Chen-Chao Xu and Wu-Zhang Yang and Wan-Li Chai and Jia-Yi Lu and Chang-Chao Liu and Bo-Sen Wang and Hao Jiang and Qian Tao and Zhi Ren and Xiao-Feng Xu and Chao Cao and Zhu-An Xu and Rui Zhou and Jin-Guang Cheng and Guang-Han Cao},
  journal= {arXiv preprint arXiv:2309.13514},
  year   = {2024}
}

Comments

32 pages, 14 figures