English

Absence of Acoustic Phonon Anomaly in a Kagome Metal with Short-ranged Structural Modulation

Strongly Correlated Electrons 2024-10-23 v1 Materials Science

Abstract

Kagome lattice AAV3_3Sb5_5 (AA = K, Rb, and Cs) superconductors without magnetism from vanadium dd-electrons are intriguing because they have a novel charge density wave (CDW) order around 90 K and display superconductivity at \sim3 K that competes with the CDW order. Recently, CsCr3_3Sb5_5, isostructural to AAV3_3Sb5_5, was found to have concurrent structural and magnetic phase transition at TT^{\ast}\approx 55 K that can be suppressed by pressure to induce superconductivity [Liu \textit{et al.}, \href{https://doi.org/10.1038/s41586-024-07761-x}{Nature \textbf{632}, 1032 (2024)}]. Here, we use elastic and inelastic X-ray scattering to study the microscopic origin of the structural transition in CsCr3_3Sb5_5. Although our elastic measurements confirm the 4×\times1×\times1 superlattice order below TT^{\ast}, its underlying correlation is rather short-ranged. Moreover, our inelastic measurements at the superlattice wavevectors around (3, 0, 0) find no evidence of a significant acoustic phonon anomaly below TT^{\ast}, similar to the case of AAV3_3Sb5_5. The absence of acoustic phonon anomaly indicates a weak electron-phonon coupling in CsCr3_3Sb5_5, suggesting that the structural transition is likely associated with an unconventional CDW order.

Keywords

Cite

@article{arxiv.2410.16465,
  title  = {Absence of Acoustic Phonon Anomaly in a Kagome Metal with Short-ranged Structural Modulation},
  author = {Weiliang Yao and Supeng Liu and Zifan Xu and Daisuke Ishikawa and Zehao Wang and Bin Gao and Sijie Xu and Feng Ye and Kenichiro Hashimoto and Takasada Shibauchi and Alfred Q. R. Baron and Pengcheng Dai},
  journal= {arXiv preprint arXiv:2410.16465},
  year   = {2024}
}

Comments

Six pages, four figures