Kagome lattice AV3Sb5 (A = K, Rb, and Cs) superconductors without magnetism from vanadium d-electrons are intriguing because they have a novel charge density wave (CDW) order around 90 K and display superconductivity at ∼3 K that competes with the CDW order. Recently, CsCr3Sb5, isostructural to AV3Sb5, was found to have concurrent structural and magnetic phase transition at T∗≈ 55 K that can be suppressed by pressure to induce superconductivity [Liu \textit{et al.}, \href{https://doi.org/10.1038/s41586-024-07761-x}{Nature \textbf{632}, 1032 (2024)}]. Here, we use elastic and inelastic X-ray scattering to study the microscopic origin of the structural transition in CsCr3Sb5. Although our elastic measurements confirm the 4×1×1 superlattice order below T∗, its underlying correlation is rather short-ranged. Moreover, our inelastic measurements at the superlattice wavevectors around (3, 0, 0) find no evidence of a significant acoustic phonon anomaly below T∗, similar to the case of AV3Sb5. The absence of acoustic phonon anomaly indicates a weak electron-phonon coupling in CsCr3Sb5, suggesting that the structural transition is likely associated with an unconventional CDW order.
@article{arxiv.2410.16465,
title = {Absence of Acoustic Phonon Anomaly in a Kagome Metal with Short-ranged Structural Modulation},
author = {Weiliang Yao and Supeng Liu and Zifan Xu and Daisuke Ishikawa and Zehao Wang and Bin Gao and Sijie Xu and Feng Ye and Kenichiro Hashimoto and Takasada Shibauchi and Alfred Q. R. Baron and Pengcheng Dai},
journal= {arXiv preprint arXiv:2410.16465},
year = {2024}
}