English

Unconventional magnetism and electronic state in frustrated layered system PdCrO$_2$

Strongly Correlated Electrons 2020-12-01 v1

Abstract

First-principles calculations and a model consideration of magnetically frustrated layered material PdCrO2_2 are performed. The results on the exchange parameters are in agreement with the experimental data on the Curie-Weiss temperature (θ\theta). We show that experimentally observed strong suppression of the N\'eel temperature (TNT_N) in comparison with the Curie-Weiss temperature is due to three main factors. First, as expected, this is connected with the layered structure and relatively small exchange interaction along the cc axis. Second, deformation of the ideal in-plane 120^{\circ} magnetic structure is crucial to provide finite TNT_N value. However, these two factors are still insufficient to explain low TNT_N and the large frustration factor θ/TN|\theta|/T_N. Thus, we suggest a scenario of an exotic non-Fermi-liquid state in PdCrO2_2 above TNT_N within the frameworks of the Anderson lattice model, which seems to explain qualitatively all its main peculiarities.

Keywords

Cite

@article{arxiv.2007.06234,
  title  = {Unconventional magnetism and electronic state in frustrated layered system PdCrO$_2$},
  author = {Evgenia V. Komleva and Valentin Yu. Irkhin and Igor V. Solovyev and Mikhail I. Katsnelson and Sergey V. Streltsov},
  journal= {arXiv preprint arXiv:2007.06234},
  year   = {2020}
}