We have used an electromigration technique to fabricate C60-based single-molecule transistors. We detail the process statistics and the protocols used to infer the successful formation of a single-molecule transistor. At low temperatures each transistor acts as a single-electron device in the Coulomb blockade regime. Resonances in the differential conductance indicate vibrational excitations consistent with a known mode of C60. In several devices we observe conductance features characteristic of the Kondo effect, a coherent many-body state comprising an unpaired spin on the molecule coupled by exchange to the conduction electrons of the leads. The inferred Kondo temperature typically exceeds 50 K, and signatures of the vibrational modes persist into the Kondo regime.
@article{arxiv.cond-mat/0310625,
title = {The Kondo effect in C$_{60}$ single-molecule transistors},
author = {L. H. Yu and D. Natelson},
journal= {arXiv preprint arXiv:cond-mat/0310625},
year = {2007}
}