English

Strong electron-phonon coupling in the sigma band of graphene

Mesoscale and Nanoscale Physics 2017-02-28 v1

Abstract

First-principles studies of the electron-phonon coupling in graphene predict a high coupling strength for the σ\sigma band with λ\lambda values of up to 0.9. Near the top of the σ\sigma band, λ\lambda is found to be 0.7\approx 0.7. This value is consistent with the recently observed kinks in the σ\sigma band dispersion by angle-resolved photoemission. While the photoemission intensity from the σ\sigma band is strongly influenced by matrix elements due to sub-lattice interference, these effects differ significantly for data taken in the first and neighboring Brillouin zones. This can be exploited to disentangle the influence of matrix elements and electron-phonon coupling. A rigorous analysis of the experimentally determined complex self-energy using Kramers-Kronig transformations further supports the assignment of the observed kinks to strong electron-phonon coupling and yields a coupling constant of 0.6(1)0.6(1), in excellent agreement with the calculations.

Keywords

Cite

@article{arxiv.1607.00939,
  title  = {Strong electron-phonon coupling in the sigma band of graphene},
  author = {Federico Mazzola and Thomas Frederiksen and Thiagarajan Balasubramanian and Philip Hofmann and Bo Hellsing and Justin W. Wells},
  journal= {arXiv preprint arXiv:1607.00939},
  year   = {2017}
}

Comments

11 pages, 3 figures