English

Phonon-induced linewidths of graphene electronic states

Materials Science 2018-12-05 v1

Abstract

The linewidths of the electronic bands originating from the electron-phonon coupling in graphene are analyzed based on model tight-binding calculations and experimental angle-resolved photoemission spectroscopy (ARPES) data. Our calculations confirm the prediction that the high-energy optical phonons provide the most essential contribution to the phonon-induced linewidth of the two upper occupied σ\sigma bands near the Γˉ\bar{\Gamma}-point. For larger binding energies of these bands, as well as for the π\pi band, we find evidence for a substantial lifetime broadening from interband scattering πσ\pi \rightarrow \sigma and σπ\sigma \rightarrow \pi, respectively, driven by the out-of-plane ZA acoustic phonons. The essential features of the calculated σ\sigma band linewidths are in agreement with recent published ARPES data [F. Mazzola et al., Phys.~Rev.~B. 95, 075430 (2017)] and of the π\pi band linewidth with ARPES data presented here.

Keywords

Cite

@article{arxiv.1808.08620,
  title  = {Phonon-induced linewidths of graphene electronic states},
  author = {B. Hellsing and T. Frederiksen and F. Mazzola and T. Balasubramanian and J. Wells},
  journal= {arXiv preprint arXiv:1808.08620},
  year   = {2018}
}

Comments

7 pages, 4 figures