English

Pseudo-Goldstone gaps and order-by-quantum-disorder in frustrated magnets

Strongly Correlated Electrons 2018-12-04 v2 Statistical Mechanics

Abstract

In systems with competing interactions, continuous degeneracies can appear which are accidental, in that they are not related to any symmetry of the Hamiltonian. Accordingly, the pseudo-Goldstone modes associated with these degeneracies are also unprotected. Indeed, through a process known as "order-by-quantum-disorder", quantum zero-point fluctuations can lift the degeneracy and induce a gap for these modes. We show that this gap can be exactly computed at leading order in 1/S1/S in spin-wave theory from the mean curvature of the classical and quantum zero-point energies - without the need to consider any spin-wave interactions. We confirm this equivalence through direct calculations of the spin-wave spectrum to O(1/S2)O(1/S^2) in a wide variety of theoretically and experimentally relevant quantum spin models. We prove this equivalence through the use of an exact sum rule that provides the required mixing of different orders of 1/S1/S. Finally, we discuss some implications for several leading order-by-quantum-disorder candidate materials, clarifying the expected pseudo-Goldstone gap sizes in Er2_2Ti2_2O7_7 and Ca3_3Fe2_2Ge3_3O12_{12}.

Keywords

Cite

@article{arxiv.1805.00947,
  title  = {Pseudo-Goldstone gaps and order-by-quantum-disorder in frustrated magnets},
  author = {Jeffrey G. Rau and Paul A. McClarty and Roderich Moessner},
  journal= {arXiv preprint arXiv:1805.00947},
  year   = {2018}
}

Comments

5 + 26 pages, 3 figures. Corrected discussion of cubic garnet, expanded supplemental material