English

Degenerate perturbation theory of quantum fluctuations in a pyrochlore antiferromagnet

Strongly Correlated Electrons 2007-05-23 v1

Abstract

We study the effect of quantum fluctuations on the half-polarized magnetization plateau of a pyrochlore antiferromagnet. We argue that an expansion around the easy axis limit is appropriate for discussing the ground state selection amongst the classically degenerate manifold of collinear states with a 3:1 ratio of spins parallel/anti-parallel to the magnetization axis. A general approach to the necessary degenerate perturbation theory is presented, and an effective quantum dimer model within this degenerate manifold is derived for arbitrary spin ss. We also generalize the existing semiclassical analysis of Hizi and Henley [Phys. Rev. B {\bf 73}, 054403 (2006)] to the easy axis limit, and show that both approaches agree at large ss. We show that under rather general conditions, the first non-constant terms in the effective Hamiltonian for s1s\geq 1 occur only at {\sl sixth} order in the transverse exchange coupling. For s3/2s\geq 3/2, the effective Hamiltonian predicts a magnetically ordered state. For s1s\leq 1 more exotic possibilities may be realized, though an analytical solution of the resulting quantum dimer model is not possible.

Keywords

Cite

@article{arxiv.cond-mat/0607210,
  title  = {Degenerate perturbation theory of quantum fluctuations in a pyrochlore antiferromagnet},
  author = {Doron L. Bergman and Ryuichi Shindou and Gregory A. Fiete and Leon Balents},
  journal= {arXiv preprint arXiv:cond-mat/0607210},
  year   = {2007}
}