English

Universal temperature-dependent power law excitation gaps in frustrated quantum spin systems harboring order-by-disorder

Strongly Correlated Electrons 2025-05-27 v1

Abstract

When magnetic moments are subject to competing or frustrated interactions, continuous degeneracies that are not protected by any symmetry of the parent Hamiltonian can emerge at the classical (mean-field) level. Such "accidental" degeneracies are often lifted by both thermal and quantum fluctuations via a mechanism known as order-by-disorder (ObD). The leading proposal to detect and characterize ObD in real materials, in a way that quantitatively distinguishes it from standard energetic selection, is to measure a small fluctuation-induced pseudo-Goldstone gap in the excitation spectrum. While the properties of this gap are known to leading order in the spin wave interactions, in both the zero-temperature and classical limits, the pseudo-Goldstone (PG) gap in quantum magnets at finite temperature has yet to be characterized. Using non-linear spin wave theory, we compute the PG gap to leading order in a 1/S1/S expansion at low temperature for a variety of frustrated quantum spin systems. We also develop a formalism to calculate the PG gap in a way that solely uses linear spin-wave theory, circumventing the need to carry out tedious quantum many-body calculations. We argue that, at leading order, the PG gap acquires a distinct power-law temperature dependence, proportional to either Td+1T^{d+1} or Td/2+1T^{d/2+1} depending on the gapless dispersion of the PG mode predicted at the mean-field level. Finally, we examine the implications of these results for the pyrochlore oxide compound Er2_2Ti2_2O7_7, for which there is compelling evidence of ObD giving rise to the experimentally observed long-range order.

Keywords

Cite

@article{arxiv.2505.18253,
  title  = {Universal temperature-dependent power law excitation gaps in frustrated quantum spin systems harboring order-by-disorder},
  author = {Alexander Hickey and Jeffrey G. Rau and Subhankar Khatua and Michel J. P. Gingras},
  journal= {arXiv preprint arXiv:2505.18253},
  year   = {2025}
}

Comments

23 pages, 5 figures