English

Proximate Spin Liquid Ground State Arising from Competing Stripy and 120$^{\circ}$ Spin Correlations in the Triangular Quantum Antiferromagnet ErMgGaO$_4$

Strongly Correlated Electrons 2026-03-11 v1

Abstract

ErMgGaO4_4 is a quantum antiferromagnet wherein the pseudospin-1/2 degrees of freedom of Er3+^{3+} decorate two-dimensional triangular planes separated by disordered non-magnetic bilayers of Mg2+^{2+} and Ga3+^{3+}. Unlike its sister compound, YbMgGaO4_4, our powder ErMgGaO4_4 sample shows a clear spin glass transition near Tg2.5T_g \sim 2.5~K, about 1/6 of its Curie-Weiss temperature. We have carried out new inelastic neutron scattering measurements on these powder ErMgGaO4_4 samples. At high energies, we observed crystalline electric field (CEF) transitions within the J=15/2J=15/2 multiplet of Er3+^{3+}, but with the first excited CEF level sufficiently low in energy (\sim 3~meV) so as to allow the possibility that virtual CEF transitions influence the exchange couplings. At E=0, we observe diffuse elastic scattering which is analysed using Warren lineshapes appropriate for two dimensional correlations. This reveals dominant 2D stripy correlations below TgT_g, coexisting with 2D 120^\circ-type correlations that persist above TgT_g. At low temperatures, the low energy inelastic component of the scattering shows a continuum with bandwidth of \sim 0.8~meV. This dynamic magnetic spectral weight can be modeled at all QQ, energies, and temperatures as the sum of high energy and low energy damped harmonic oscillators (DHO), with the high energy DHO defining the bandwidth of \sim 0.8~meV. We use linear spin wave theory to model this inelastic scattering and to estimate its spin Hamiltonian parameters in terms of a J1J2ΔJ_1-J_2-\Delta model on the triangular lattice. This gives a good description of the low lying spectral weight for ErMgGaO4, and allows us to place it on the theoretical J1J2ΔJ_1-J_2-\Delta phase diagram with J1J2=0.13±0.03\frac{J_1}{J_2}=0.13 \pm 0.03 and Δ=0.4±0.1\Delta=0.4 \pm 0.1, which is close to the expected quantum phase boundary between the spin liquid and the stripy ordered phases.

Keywords

Cite

@article{arxiv.2603.08934,
  title  = {Proximate Spin Liquid Ground State Arising from Competing Stripy and 120$^{\circ}$ Spin Correlations in the Triangular Quantum Antiferromagnet ErMgGaO$_4$},
  author = {S. H. -Y. Huang and S. Petit and Bo Yuan and Z. W. Cronkwright and C. Pinvidic and Y. Wang and E. M. Smith and S. Bhattacharya and C. Yang and J. -M. Zanotti and Q. Berrod and M. B. Stone and A. I. Kolesnikov and R. J. Cava and E. Kermarrec and B. D. Gaulin},
  journal= {arXiv preprint arXiv:2603.08934},
  year   = {2026}
}

Comments

20 pages, 19 figures, abstract slightly modified to meet Arxiv character requirement; see PDF for full abstract