Proximate Spin Liquid Ground State Arising from Competing Stripy and 120$^{\circ}$ Spin Correlations in the Triangular Quantum Antiferromagnet ErMgGaO$_4$
Abstract
ErMgGaO is a quantum antiferromagnet wherein the pseudospin-1/2 degrees of freedom of Er decorate two-dimensional triangular planes separated by disordered non-magnetic bilayers of Mg and Ga. Unlike its sister compound, YbMgGaO, our powder ErMgGaO sample shows a clear spin glass transition near ~K, about 1/6 of its Curie-Weiss temperature. We have carried out new inelastic neutron scattering measurements on these powder ErMgGaO samples. At high energies, we observed crystalline electric field (CEF) transitions within the multiplet of Er, but with the first excited CEF level sufficiently low in energy ( 3~meV) so as to allow the possibility that virtual CEF transitions influence the exchange couplings. At E=0, we observe diffuse elastic scattering which is analysed using Warren lineshapes appropriate for two dimensional correlations. This reveals dominant 2D stripy correlations below , coexisting with 2D 120-type correlations that persist above . At low temperatures, the low energy inelastic component of the scattering shows a continuum with bandwidth of 0.8~meV. This dynamic magnetic spectral weight can be modeled at all , energies, and temperatures as the sum of high energy and low energy damped harmonic oscillators (DHO), with the high energy DHO defining the bandwidth of 0.8~meV. We use linear spin wave theory to model this inelastic scattering and to estimate its spin Hamiltonian parameters in terms of a model on the triangular lattice. This gives a good description of the low lying spectral weight for ErMgGaO4, and allows us to place it on the theoretical phase diagram with and , which is close to the expected quantum phase boundary between the spin liquid and the stripy ordered phases.
Keywords
Cite
@article{arxiv.2603.08934,
title = {Proximate Spin Liquid Ground State Arising from Competing Stripy and 120$^{\circ}$ Spin Correlations in the Triangular Quantum Antiferromagnet ErMgGaO$_4$},
author = {S. H. -Y. Huang and S. Petit and Bo Yuan and Z. W. Cronkwright and C. Pinvidic and Y. Wang and E. M. Smith and S. Bhattacharya and C. Yang and J. -M. Zanotti and Q. Berrod and M. B. Stone and A. I. Kolesnikov and R. J. Cava and E. Kermarrec and B. D. Gaulin},
journal= {arXiv preprint arXiv:2603.08934},
year = {2026}
}
Comments
20 pages, 19 figures, abstract slightly modified to meet Arxiv character requirement; see PDF for full abstract