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The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

The spin-1/2 triangular lattice antiferromagnet YbMgGaO$_{4}$ has attracted recent attention as a quantum spin-liquid candidate with the possible presence of off-diagonal anisotropic exchange interactions induced by spin-orbit coupling.…

We present a detailed magnetic study of the triangular antiferromagnet ErMgGaO$_4$. A point charge calculation under the single ion approximation reveals a crystal field ground state doublet with a strong Ising-like behavior of the…

Strongly Correlated Electrons · Physics 2020-04-08 Y. Cai , C. Lygouras , G. Thomas , M. N. Wilson , J. Beare , D. R. Yahne , K. Ross , Z. Gong , Y. J. Uemura , H. A. Dabkowska , G. M. Luke

The transverse-field Ising model on the triangular lattice is expected to host an intermediate finite-temperature Kosterlitz-Thouless (KT) phase through a mapping of the spins on each triangular unit to a complex order parameter.…

DC-magnetization data measured down to 40 mK speak against conventional freezing and reinstate YbMgGaO$_4$ as a triangular spin-liquid candidate. Magnetic susceptibility measured parallel and perpendicular to the $c$-axis reaches constant…

We present a neutron triple-axis and resonant spin-echo spectroscopy study of the spin correlations in untwinned YBCO crystals with x= 0.3, 0.35, and 0.45 as a function of temperature and magnetic field. As the temperature T approaches 0,…

Strongly Correlated Electrons · Physics 2015-05-19 D. Haug , V. Hinkov , Y. Sidis , P. Bourges , N. B. Christensen , A. Ivanov , T. Keller , C. T. Lin , B. Keimer

We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state…

LuCuGaO4 has magnetic Cu2+ and diamagnetic Ga3+ ions distributed on a triangular bilayer and is suggested to undergo a spin-glass transition with T_g approximately 0.4 K. Using muSR and neutron scattering measurements, we show that at low…

Materials Science · Physics 2013-05-29 S Calder , SR Giblin , DR Parker , PP Deen , C Ritter , JR Stewart , S Rols , T Fennell

YbMgGaO$_{4}$, a structurally perfect two-dimensional triangular lattice with odd number of electrons per unit cell and spin-orbit entangled effective spin-1/2 local moments of Yb$^{3+}$ ions, is likely to experimentally realize the quantum…

Strongly Correlated Electrons · Physics 2015-10-20 Yuesheng Li , Gang Chen , Wei Tong , Li Pi , Juanjuan Liu , Zhaorong Yang , Xiaoqun Wang , Qingming Zhang

We report magnetization, heat capacity, thermal expansion, and magnetostriction measurements down to millikelvin temperatures on the triangular antiferromagnet YbMgGaO$_4$. Our data exclude the formation of the distinct $\frac13$ plateau…

$^{51}$V NMR studies on CaV2O4 single crystals and $^{17}$O NMR studies on $^{17}$O-enriched powder samples are reported. The temperature dependences of the $^{17}$O NMR line width and nuclear spin-lattice relaxation rate give strong…

Strongly Correlated Electrons · Physics 2010-11-17 X. Zong , B. J. Suh , A. Niazi , J. Q. Yan , D. L. Schlagel , T. A. Lograsso , D. C. Johnston

The A-site ordered chromate spinels LiGa1-xInxCr4O8 host a network of size-alternating spin-3/2 Cr3+ tetrahedra known as a 'breathing' pyrochlore lattice. For the x=0.05 composition, the complex magneto-structural ordering observed in the…

Motivated by the recent experiment on a rare-earth material YbMgGaO$_4$ [Y. Li \textit{et al.}, Phys. Rev. Lett. \textbf{115}, 167203 (2015)], which found that the ground state of YbMgGaO$_4$ is a quantum spin liquid, we study the…

Strongly Correlated Electrons · Physics 2017-04-26 Qiang Luo , Shijie Hu , Bin Xi , Jize Zhao , Xiaoqun Wang

Neutron scattering is used to investigate spin correlations in ultra pure single crystals of the S=1 triangular lattice NiGa2S4. Despite a Curie-Weiss temperature of Theta_CW=-80(2) K, static (tau > 1 ns) short range (xi_ab=26(3) \AA)…

Strongly Correlated Electrons · Physics 2015-05-19 C. Stock , S. Jonas , C. Broholm , S. Nakatsuji , Y. Nambu , K. Onuma , Y. Maeno , J. -H. Chung

Elastic and inelastic neutron scattering studies reveal details of the antiferromagnetic tansition and intriguing spin-dynamics in the magneto-electric effect single crystal LiMnPO$_4$. The elastic scattering studies confirm the system is…

Strongly Correlated Electrons · Physics 2015-05-13 Jiying Li , Wei Tian , Ying Chen , Jerel L. Zarestky , Jeffrey W. Lynn , David Vaknin

Spin-wave dispersions in the antiferromagnetic state of single crystal LiFePO$_4$ were determined by inelastic neutron scattering measurements. The dispersion curves measured from the (010) reflection along both {\it a}$^\ast$ and {\it…

Materials Science · Physics 2009-11-11 Jiying Li , Vasile O. Garlea , Jerel L. Zarestky , David Vaknin

By performing time-of-flight neutron scattering measurements on a large amount of single crystals of Sr$_2$RuO$_4$, we studied detailed structure of the imaginary part of the dynamic spin susceptibility over a wide range of phase space. In…

Strongly Correlated Electrons · Physics 2015-05-28 K. Iida , M. Kofu , N. Katayama , J. Lee , R. Kajimoto , Y. Inamura , M. Nakamura , M. Arai , Y. Yoshida , M. Fujita , K. Yamada , S. -H. Lee

The pyrochlore material Yb2Ti2O7 displays unexpected quasi-two-dimensional (2D) magnetic correlations within a cubic lattice environment at low temperatures, before entering an exotic disordered ground state below T=265mK. We report neutron…

Strongly Correlated Electrons · Physics 2012-02-13 K. A. Ross , L. R. Yaraskavitch , M. Laver , J. S. Gardner , J. A. Quilliam , S. Meng , J. B. Kycia , D. K. Singh , H. A. Dabkowska , B. D. Gaulin

Magnetic order on the spatially anisotropic triangular lattice of $\alpha$-NaMnO$_2$ is studied via neutron diffraction measurements. The transition into a commensurate, collinear antiferromagnetic ground state with $\mathbf{k}=(0.5, 0.5,…

Strongly Correlated Electrons · Physics 2018-11-14 Rebecca L. Dally , Robin Chisnell , Leland Harriger , Yaohua Liu , Jeffrey W. Lynn , Stephen D. Wilson

The quantum spin liquid (QSL) state is an exotic state of matter featuring a high degree of entanglement and lack of long-range magnetic order in the zero-temperature limit. The triangular antiferromagnet YbMgGaO4 is a candidate QSL host,…

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