English

Phonon-Mediated Quasiparticle Lifetime Renormalizations in Few-Layer Hexagonal Boron Nitride

Materials Science 2023-08-29 v1

Abstract

Understanding the collective behavior of the quasiparticles in solid-state systems underpins the field of non-volatile electronics, including the opportunity to control many-body effects for well-desired physical phenomena and their applications. Hexagonal boron nitride (hBN) is a wide energy bandgap semiconductor, showing immense potential as a platform for low-dimensional device heterostructures. It is an inert dielectric used for gated devices, having a negligible orbital hybridization when placed in contact with other systems. Despite its inertness, we discover a large electron mass enhancement in few-layer hBN affecting the lifetime of the π\pi-band states. We show that the renormalization is phonon-mediated and consistent with both single- and multiple-phonon scattering events. Our findings thus unveil a so-far unknown many-body state in a wide-bandgap insulator, having important implications for devices using hBN as one of their building blocks.

Keywords

Cite

@article{arxiv.2308.13846,
  title  = {Phonon-Mediated Quasiparticle Lifetime Renormalizations in Few-Layer Hexagonal Boron Nitride},
  author = {Håkon I. Røst and Simon P. Cooil and Anna Cecilie Åsland and Jinbang Hu and Ayaz Ali and Takashi Taniguchi and Kenji Watanabe and Branson D. Belle and Bodil Holst and Jerzy T. Sadowski and Federico Mazzola and Justin W. Wells},
  journal= {arXiv preprint arXiv:2308.13846},
  year   = {2023}
}

Comments

This document is the unedited Author's version of a Submitted Work that was subsequently accepted for publication in Nano Letters, copyright $\copyright$ 2022 The Authors, licensed under CC-BY 4.0 after peer review. To access the final edited and published work see https://doi.org/10.1021/acs.nanolett.3c02086

R2 v1 2026-06-28T12:05:00.123Z