English

Phase-ordering kinetics in the Allen-Cahn (Model A) class: universal aspects elucidated by electrically-induced transition in liquid crystals

Statistical Mechanics 2024-03-14 v3 Soft Condensed Matter

Abstract

The two-dimensional (2d) Ising model is the statistical physics textbook example for phase transitions and their kinetics. Quenched through the Curie point with Glauber rates, the late-time description of the ferromagnetic domain coarsening finds its place at the scalar sector of the Allen-Cahn (Model A) class. Resisting exact results sought since Lifshitz's account in 1962, central quantities in 2d Model A - most scaling exponents and correlation functions - remain known up to approximate theories whose disparate outcomes urge experimental assessment. Here, we perform such assessment from a comprehensive study of the coarsening of 2d twisted nematic liquid crystals whose kinetics is induced by a super-fast switching from a spatiotemporally chaotic state to a two-phase concurrent, equilibrium one. Tracking the dynamics via optical microscopy, we firstly show the sharp evidence of well-established Model A aspects, such as the dynamic exponent z=2z=2 and the dynamic scaling hypothesis, to then move forward. We confirm the Bray-Humayun theory for Porod's regime describing intradomain length scales of spatial correlators, and show that their nontrivial decay beyond that regime is captured in a free-from-parameter fashion by Gaussian theories. These paradigmatic theories, however, do not perform well for time-related Model A statistics. We reveal that the collapsed form of two-time correlators is best accounted for by the local scaling invariance theory, along with the Fisher-Huse conjecture. We also suggest the true value for the local persistence exponent, in disfavour of Gaussian models, and extract a universal fractal dimension for the morphology of persistence clusters that is notably close to the golden ratio. Given its accuracy and possibilities, this experimental setup may work as a prototype to address universality issues in the realm of nonequilibrium systems.

Keywords

Cite

@article{arxiv.2107.09043,
  title  = {Phase-ordering kinetics in the Allen-Cahn (Model A) class: universal aspects elucidated by electrically-induced transition in liquid crystals},
  author = {Renan A. L. Almeida and Kazumasa A. Takeuchi},
  journal= {arXiv preprint arXiv:2107.09043},
  year   = {2024}
}

Comments

19 pages, 10 figures, 2 tables