English

Persistent spin dynamics in the pressurized spin-liquid candidate YbMgGaO$_4$

Strongly Correlated Electrons 2020-05-20 v2 Materials Science

Abstract

Single-crystal x-ray diffraction, density-functional band-structure calculations, and muon spin relaxation (μ\muSR) are used to probe pressure evolution of the triangular spin-liquid candidate YbMgGaO4_4. The rhombohedral crystal structure is retained up to at least 10 GPa and shows a nearly uniform compression along both in-plane and out-of-plane directions, whereas local distortions caused by the random distribution of Mg2+^{2+} and Ga3+^{3+} remain mostly unchanged. The μ\muSR data confirm persistent spin dynamics up to 2.6 GPa and down to 250 mK with no change in the muon relaxation rate. Longitudinal-field μ\muSR reveals power-law behavior of the spin-spin autocorrelation function, both at ambient pressure and upon compression.

Keywords

Cite

@article{arxiv.1902.07749,
  title  = {Persistent spin dynamics in the pressurized spin-liquid candidate YbMgGaO$_4$},
  author = {Mayukh Majumder and Gediminas Simutis and Ines E. Collings and Jean-Christophe Orain and Tusharkanti Dey and Yuesheng Li and Philipp Gegenwart and Alexander A. Tsirlin},
  journal= {arXiv preprint arXiv:1902.07749},
  year   = {2020}
}

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published version

R2 v1 2026-06-23T07:46:26.115Z