English

Metastable antiphase boundary ordering in CaFe$_{2}$O$_{4}$

Strongly Correlated Electrons 2021-09-14 v2

Abstract

CaFe2_{2}O4_{4} is an S=5/2S=5/2 antiferromagnet exhibiting two magnetic orders which shows regions of coexistence at some temperatures. Using a Green's function formalism, we model neutron scattering data of the spin wave excitations in this material, ellucidating the microscopic spin Hamiltonian. In doing so, we suggest that the low temperature A phase order ()(\uparrow\uparrow\downarrow\downarrow) finds its origins in the freezing of antiphase boundaries created by thermal fluctuations in a parent B phase order ()(\uparrow\downarrow\uparrow\downarrow). The low temperature magnetic order observed in CaFe2_{2}O4_{4} is thus the result of a competition between the exchange coupling along cc, which favors the B phase, and the single-ion anisotropy which stabilizes thermally-generated antiphase boundaries, leading to static metastable A phase order at low temperatures.

Keywords

Cite

@article{arxiv.2108.09679,
  title  = {Metastable antiphase boundary ordering in CaFe$_{2}$O$_{4}$},
  author = {H. Lane and E. E. Rodriguez and H. C. Walker and Ch. Niedermayer and U. Stuhr and R. I. Bewley and D. J. Voneshen and M. A. Green and J. A. Rodriguez-Rivera and P. Fouquet and S. -W. Cheong and J. P. Attfield and R. A. Ewings and C. Stock},
  journal= {arXiv preprint arXiv:2108.09679},
  year   = {2021}
}

Comments

16 pages, 10 figures

R2 v1 2026-06-24T05:19:04.795Z