English

beta-Cu3V2O8: Magnetic ordering in a spin-1/2 kagome-staircase lattice

Condensed Matter 2012-08-16 v1

Abstract

The spin-1/2 Cu2+ ions in beta-Cu3V2O8 occupy the sites of a Kagome-staircase lattice, an anisotropic variant of the Kagome net: buckled layers and imbedded plaquettes of three edge-shared CuO4 squares break the ideal Kagome symmetry. Susceptibility and heat capacity measurements show the onset of short-range ordering at approximately 75 K, and a magnetic phase transition with the characteristics of antiferromagnetism at ~29 K. Comparison to the Curie Weiss theta (theta,CW = -135 K) indicates that the geometric frustration is largely relieved by the anisotropy. A ferromagnetic contribution to the magnetization below the ordering temperature and negative magnetization in zero-field cooled measurements at low fields are attributed to uncompensated spins at grain boundaries or defects.

Keywords

Cite

@article{arxiv.cond-mat/0211573,
  title  = {beta-Cu3V2O8: Magnetic ordering in a spin-1/2 kagome-staircase lattice},
  author = {N. Rogado and M. K. Haas and G. Lawes and D. A. Huse and A. P. Ramirez and R. J. Cava},
  journal= {arXiv preprint arXiv:cond-mat/0211573},
  year   = {2012}
}

Comments

9 pages, 5 figures