English

Lateral Exchange Bias for N\'eel-Vector Control in Atomically Thin Antiferromagnets

Materials Science 2025-08-21 v2 Mesoscale and Nanoscale Physics

Abstract

Atomically thin van der Waals (vdW) magnets have emerged as a fascinating platform for the exploration of novel physical phenomena arising from their reduced dimensionality and exceptional material properties. Their single-crystalline nature and ultimate miniaturization position them as leading candidates for next-generation spintronic applications. Antiferromagnetic (AF) vdW magnets are of particular interest, as they combine the advantages of vdW magnets with the functionality of AF spintronics, offering unique opportunities for ultrafast and robust spintronic devices. However, the lack of approaches to locally and deterministically manipulate their order parameter -- the N\'eel-vector -- remains a key limitation. Here, we introduce a fundamentally new paradigm in nanomagnetism, which we term lateral exchange bias (LEB), to achieve N\'eel vector control in bilayers of the vdW AF CrSBr. We exploit the single-crystalline registry formed by terraced CrSBr samples, where the bilayer N\'eel vector is controlled by LEB from neighboring, odd-layered flakes, whose nonzero magnetization we manipulate using magnetic fields. Using this control, we achieve nonvolatile manipulation of magnetic domains and domain walls (DWs) in AF CrSBr bilayers, establishing a powerful toolkit for controlling atomically thin AFs at the nanoscale. Our results challenge conventional views on exchange bias and provide a previously unexplored mechanism for achieving atomic-scale control of AFic order. Our findings pave the way for the development of advanced spintronic architectures and quantum technologies based on vdW magnets.

Keywords

Cite

@article{arxiv.2503.04922,
  title  = {Lateral Exchange Bias for N\'eel-Vector Control in Atomically Thin Antiferromagnets},
  author = {Clément Pellet-Mary and Debarghya Dutta and Märta A. Tschudin and Patrick Siegwolf and Boris Gross and David A. Broadway and Jordan Cox and Carolin Schrader and Jodok Happacher and Daniel G. Chica and Cory R. Dean and Xavier Roy and Patrick Maletinsky},
  journal= {arXiv preprint arXiv:2503.04922},
  year   = {2025}
}
R2 v1 2026-06-28T22:09:58.047Z