English

Electronic correlations in the van der Waals ferromagnet Fe$_3$GeTe$_2$ revealed by its charge dynamics

Strongly Correlated Electrons 2020-12-02 v1

Abstract

The layered van der Waals ferromagnetic Fe3_3GeTe2_2 harbours an unconventional interplay between topology and magnetism, leading to a large anomalous Hall conductivity at low temperatures. Here, we investigate the temperature dependence of its charge dynamics and reveal that upon entering the ferromagnetic state at TC200T_C \sim 200 K and further lowering the temperature there is the onset of a gradual spectral weight reshuffling from the mid-infrared range towards far- as well as near-infrared frequencies. This two-fold spectral weight transfer indicates the important role of the Hund's coupling as primary source for electronic correlations and signals an incoherent-coherent crossover at low temperatures. Our findings also convey the electronic environment, based on nodal-line topological states, favouring the large anomalous Hall conductivity.

Keywords

Cite

@article{arxiv.2010.02662,
  title  = {Electronic correlations in the van der Waals ferromagnet Fe$_3$GeTe$_2$ revealed by its charge dynamics},
  author = {M. Corasaniti and R. Yang and K. Sen and K. Willa and M. Merz and A. A. Haghighirad and M. Le Tacon and L. Degiorgi},
  journal= {arXiv preprint arXiv:2010.02662},
  year   = {2020}
}

Comments

6 pages, 3 figures, Phys. Rev. B (Rapid Communication), in press