Fe3GaTe2, a recently discovered van der Waals ferromagnet, demonstrates intrinsic ferromagnetism above room temperature, necessitating a comprehensive investigation of the microscopic origins of its high Curie temperature (TC). In this study, we reveal the electronic structure of Fe3GaTe2 in its ferromagnetic ground state using angle-resolved photoemission spectroscopy and density functional theory calculations. Our results establish a consistent correspondence between the measured band structure and theoretical calculations, underscoring the significant contributions of the Heisenberg exchange interaction (Jex) and magnetic anisotropy energy to the development of the high-TC ferromagnetic ordering in Fe3GaTe2. Intriguingly, we observe substantial modifications to these crucial driving factors through doping, which we attribute to alterations in multiple spin-splitting bands near the Fermi level. These findings provide valuable insights into the underlying electronic structure and its correlation with the emergence of high-TC ferromagnetic ordering in Fe3GaTe2.
@article{arxiv.2403.09846,
title = {Electronic structure of above-room-temperature van der Waals ferromagnet Fe$_3$GaTe$_2$},
author = {Ji-Eun Lee and Shaohua Yan and Sehoon Oh and Jinwoong Hwang and Jonathan D. Denlinger and Choongyu Hwang and Hechang Lei and Sung-Kwan Mo and Se Young Park and Hyejin Ryu},
journal= {arXiv preprint arXiv:2403.09846},
year = {2024}
}