English

Electronic structure of above-room-temperature van der Waals ferromagnet Fe$_3$GaTe$_2$

Materials Science 2024-03-18 v1

Abstract

Fe3_3GaTe2_2, a recently discovered van der Waals ferromagnet, demonstrates intrinsic ferromagnetism above room temperature, necessitating a comprehensive investigation of the microscopic origins of its high Curie temperature (T\textit{T}C_C). In this study, we reveal the electronic structure of Fe3_3GaTe2_2 in its ferromagnetic ground state using angle-resolved photoemission spectroscopy and density functional theory calculations. Our results establish a consistent correspondence between the measured band structure and theoretical calculations, underscoring the significant contributions of the Heisenberg exchange interaction (J\textit{J}ex_{ex}) and magnetic anisotropy energy to the development of the high-T\textit{T}C_C ferromagnetic ordering in Fe3_3GaTe2_2. Intriguingly, we observe substantial modifications to these crucial driving factors through doping, which we attribute to alterations in multiple spin-splitting bands near the Fermi level. These findings provide valuable insights into the underlying electronic structure and its correlation with the emergence of high-T\textit{T}C_C ferromagnetic ordering in Fe3_3GaTe2_2.

Keywords

Cite

@article{arxiv.2403.09846,
  title  = {Electronic structure of above-room-temperature van der Waals ferromagnet Fe$_3$GaTe$_2$},
  author = {Ji-Eun Lee and Shaohua Yan and Sehoon Oh and Jinwoong Hwang and Jonathan D. Denlinger and Choongyu Hwang and Hechang Lei and Sung-Kwan Mo and Se Young Park and Hyejin Ryu},
  journal= {arXiv preprint arXiv:2403.09846},
  year   = {2024}
}

Comments

25 pages, 4 figures