English

Electronic and magnetic properties of graphene quantum dots with two charged vacancies

Mesoscale and Nanoscale Physics 2020-08-21 v2

Abstract

Electronic and magnetic properties of a system of two charged vacancies in hexagonal shaped graphene quantum dots are investigated using a mean-field Hubbard model as a function of the Coulomb potential strength β\beta of the charge impurities and the distance R between them. For β=0\beta=0, the magnetic properties of the vacancies are dictated by Lieb's rules where the opposite (same) sub-lattice vacancies are coupled antiferromagnetically (ferromagnetically) and exhibit Fermi oscillations. Here, we demonstrate the emergence of a non-magnetic regime within the subcritical region: as the Coulomb potential strength is increased to β0.1\beta \sim 0.1 , before reaching the frustrated atomic collapse regime, the magnetization is strongly suppressed and the ground state total spin is given by Sz=0S_{z}=0 both for opposite and same sublattice vacancy configurations. When long-range electron-electronz in-teractions are included within extended mean-field Hubbard model, the critical value for the frustrated collapse increases from βcf0.28\beta_{cf} \sim 0.28 to βcf0.36\beta_{cf} \sim 0.36 for R<27 A˚R < 27 \ \r{A} .

Keywords

Cite

@article{arxiv.2006.11048,
  title  = {Electronic and magnetic properties of graphene quantum dots with two charged vacancies},
  author = {E. Bulut Kul and M. Polat and A. D. Güçlü},
  journal= {arXiv preprint arXiv:2006.11048},
  year   = {2020}
}

Comments

8 pages, 5 figures